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Instrumentation and measurement strategy for the NOAA SENEX aircraft campaign as part of the Southeast Atmosphere Study 2013

Authors :
Joel A. Thornton
David W. Fahey
Kenneth C. Aikin
Kyung-Eun Min
Michael Trainer
Carsten Warneke
James M. Roberts
Nicholas L. Wagner
Thomas B. Ryerson
Jingqiu Mao
Milos Z. Markovic
Courtney D. Hatch
Frank N. Keutsch
Thomas F. Hanisco
J. Kaiser
Patrick R. Veres
Glenn M. Wolfe
Joost A. de Gouw
J. A. Neuman
William P. Dubé
Felipe D. Lopez-Hilfiker
Martin Graus
Steven S. Brown
Ravan Ahmadov
Rebecca A. Washenfelder
Jack J. Lin
T. D. Gordon
Joshua P. Schwarz
Aikaterini Bougiatioti
John B. Nowak
Daniel Law
Peter Edwards
Jessica B. Gilman
Ann M. Middlebrook
Mathew Richardson
Ben H. Lee
Jin Liao
Athanasios Nenes
Brian M. Lerner
John S. Holloway
Jeff Peischl
Daniel A. Lack
David D. Parrish
Steven Sjostedt
André Welti
A. R. Ravishankara
Iliana Pollack
Stuart A. McKeen
Gerhard Hübler
Charles A. Brock
Jerome Brioude
Cooperative Institute for Research in Environmental Sciences (CIRES)
University of Colorado [Boulder]-National Oceanic and Atmospheric Administration (NOAA)
NOAA Earth System Research Laboratory (ESRL)
National Oceanic and Atmospheric Administration (NOAA)
Laboratoire de l'Atmosphère et des Cyclones (LACy)
Centre National de la Recherche Scientifique (CNRS)-Université de La Réunion (UR)-Institut national des sciences de l'Univers (INSU - CNRS)-Météo France
Georgia Institute of Technology [Atlanta]
Foundation for Research and Technology - Hellas (FORTH)
National Observatory of Athens (NOA)
NASA Goddard Space Flight Center (GSFC)
University of Maryland [Baltimore County] (UMBC)
University of Maryland System
University of Washington [Seattle]
University of Wisconsin-Madison
NOAA Geophysical Fluid Dynamics Laboratory (GFDL)
Princeton University
Hendrix College
Source :
Atmospheric Measurement Techniques, Atmospheric Measurement Techniques, European Geosciences Union, 2016, 9, pp.3063-3093. ⟨10.5194/amt-9-3063-2016⟩, Atmospheric Measurement Techniques, Vol 9, Iss 7, Pp 3063-3093 (2016)
Publication Year :
2018

Abstract

The Southeast United States (US) might not have warmed as much as the rest of the country over the past 50-100 years. Providing an improved understanding of this potential anomaly, and specifically the roles played by aerosols, was one of the main goals for the Southeast Atmosphere Study (SAS). Natural emissions of ozone-and-aerosol-precursor gases such as isoprene and monoterpenes are high in the southeast of the US. In addition, anthropogenic emissions are significant inthe Southeast US and summertime photochemistry is rapid. The NOAA-led SENEX (Southeast Nexus) aircraft campaign was one of the major components of the SAS studyand was focused on studying the interactions between biogenic and anthropogenic emissions to form secondary pollutants. During SENEX, the NOAA WP-3D aircraft conducted 20 research flights between 27 May and 10 July 2013 based out of Smyrna, TN. Here we describe the experimental approach, the science goals and early results of the NOAA SENEX campaign. The aircraft, its capabilities and standard measurements are described. The instrument payload is summarized including detection limits, accuracy, precision and time resolutions for all gas-and-aerosol phase instruments. The inter-comparisons of compounds measured with multiple instruments on the NOAA WP-3D are presented and were almost all within the stated uncertainties. The SENEX flights included day- and nighttime flights in the Southeast as well as flights over areas with intense shale gas extraction (Marcellus, Fayetteville and Haynesville shale). We present one example flight on 16 June 2013, which was a daytime flight over the Atlanta region, where several crosswind transects of plumes from the city and nearby point sources, such as power plants, paper mills and landfills, were flown. The area around Atlanta has large biogenic isoprene emissions, which provided an excellent case for studying the interactions between biogenic and anthropogenic emissions. In this example flight, chemistry in and outside the Atlanta plumes was observed for several hours after emission. The analysis of this flight showcases the strategies implemented to answer some of the main SENEX science questions.

Details

Language :
English
ISSN :
18678548 and 18671381
Database :
OpenAIRE
Journal :
Atmospheric Measurement Techniques, Atmospheric Measurement Techniques, European Geosciences Union, 2016, 9, pp.3063-3093. ⟨10.5194/amt-9-3063-2016⟩, Atmospheric Measurement Techniques, Vol 9, Iss 7, Pp 3063-3093 (2016)
Accession number :
edsair.doi.dedup.....4c3d8820018ba3eb9fe7c64b40754a6a