Evidence for Magnetic Field Induced Changes of the Phase of Tunneling States: Spontaneous Echoes in (KBr)$_{1-x}$(KCN)$_x$ in Magnetic Fields

Recently, it has been discovered that in contrast to expectations the low-temperature dielectric properties of some multi-component glasses depend strongly on magnetic fields. In particular, the low-frequency dielectric susceptibility and the amplitude of coherent polarization echoes show striking non-monotonic magnetic field dependencies. The low-temperature dielectric response of these materials is governed by atomic tunneling systems. We now have investigated the coherent properties of tunneling states in a crystalline host in magnetic fields up to 230$ $mT. Two-pulse echo experiments have been performed on a KBr crystal containing about 7.5% CN$^-$. Like in glasses, but perhaps even more surprising in the case of a crystalline system, we observe a very strong magnetic field dependence of the echo amplitude. Moreover, for the first time we have direct evidence that magnetic fields change the phase of coherent tunneling systems in a well-defined way. We present the data and discuss the possible origin of this intriguing effect.
Comment: 4 pages, 3 figures, submitted to PRL