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Ammonia-assisted fast Li-ion conductivity in a new hemiammine lithium borohydride, LiBH4·1/2NH3

Authors :
Young-Su Lee
Yigang Yan
Young Whan Cho
Jakob B. Grinderslev
Mathias Jørgensen
Radovan Černý
Torben R. Jensen
Source :
Chemical Communications, Vol. 56, No 28 (2020) pp. 3971-3974, Yan, Y, Grinderslev, J B, Lee, Y S, Jørgensen, M, Cho, Y W, Černý, R & Jensen, T R 2020, ' Ammonia-assisted fast Li-ion conductivity in a new hemiammine lithium borohydride, LiBH 4 ·1/2NH 3 ', Chemical Communications, vol. 56, no. 28, pp. 3971-3974 . https://doi.org/10.1039/c9cc09990e
Publication Year :
2020

Abstract

Hemiammine lithium borohydride, LiBH4·1/2NH3, is characterized and a new Li+ conductivity mechanism is identified. It exhibits a Li+ conductivity of 7 × 10-4 S cm-1 at 40 °C in the solid state and 3.0 × 10-2 S cm-1 at 55 °C after melting. The molten state of LiBH4·1/2NH3 has a high viscosity and can be mechanically stabilized in nano-composites with inert metal oxides and other hydrides making it a promising battery electrolyte.

Details

Language :
English
ISSN :
13597345
Database :
OpenAIRE
Journal :
Chemical Communications, Vol. 56, No 28 (2020) pp. 3971-3974, Yan, Y, Grinderslev, J B, Lee, Y S, Jørgensen, M, Cho, Y W, Černý, R & Jensen, T R 2020, ' Ammonia-assisted fast Li-ion conductivity in a new hemiammine lithium borohydride, LiBH 4 ·1/2NH 3 ', Chemical Communications, vol. 56, no. 28, pp. 3971-3974 . https://doi.org/10.1039/c9cc09990e
Accession number :
edsair.doi.dedup.....598870aaf3fb873c95cba7219f9c2a50
Full Text :
https://doi.org/10.1039/c9cc09990e