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Thermoelectric Conversion at 30 K in InAs/InP Nanowire Quantum Dots

Authors :
Fabio Taddei
Fabio Beltram
Domenic Prete
Lucia Sorba
Valentina Zannier
Paolo Andrea Erdman
Francesco Rossella
Daniele Ercolani
Valeria Demontis
Stefano Roddaro
Prete, D.
Erdman, P. A.
Demontis, V.
Zannier, V.
Ercolani, D.
Sorba, L.
Beltram, F.
Rossella, F.
Taddei, F.
Roddaro, S.
Source :
Nano letters, 19 (2019): 3033–3039. doi:10.1021/acs.nanolett.9b00276, info:cnr-pdr/source/autori:Prete D.; Erdman P.A.; Demontis V.; Zannier V.; Ercolani D.; Sorba L.; Beltram F.; Rossella F.; Taddei F.; Roddaro S./titolo:Thermoelectric Conversion at 30 K in InAs%2FInP Nanowire Quantum Dots/doi:10.1021%2Facs.nanolett.9b00276/rivista:Nano letters (Print)/anno:2019/pagina_da:3033/pagina_a:3039/intervallo_pagine:3033–3039/volume:19
Publication Year :
2019

Abstract

We demonstrate high-temperature thermoelectric conversion in InAs/InP nanowire quantum dots by taking advantage of their strong electronic confinement. The electrical conductance G and the thermopower S are obtained from charge transport measurements and accurately reproduced with a theoretical model accounting for the multi-level structure of the quantum dot. Notably, our analysis does not rely on the estimate of co-tunnelling contributions since electronic thermal transport is dominated by multi-level heat transport. By taking into account two spin-degenerate energy levels we are able to evaluate the electronic thermal conductance K and investigate the evolution of the electronic figure of merit ZT as a function of the quantum dot configuration and demonstrate ZT ~ 35 at 30 K, corresponding to an electronic effciency at maximum power close to the Curzon- Ahlborn limit.<br />7 pages, 4 figures

Details

ISSN :
15306992
Volume :
19
Issue :
5
Database :
OpenAIRE
Journal :
Nano letters
Accession number :
edsair.doi.dedup.....5a61d4a74e2b4360dba31e3b6f082b2d
Full Text :
https://doi.org/10.1021/acs.nanolett.9b00276