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Enhanced passivity of Cr-Fe-Co-Ni-Mo multi-component single-phase face-centred cubic alloys: design, production and corrosion behaviour

Authors :
Wang, Xueying
Mercier, Dimitri
Danard, Yolande
Rieger, Thomas
Perrière, Loïc
Laurent-Brocq, Mathilde
Guillot, Ivan
Maurice, Vincent
Marcus, Philippe
Institut de Recherche de Chimie Paris (IRCP)
Ecole Nationale Supérieure de Chimie de Paris - Chimie ParisTech-PSL (ENSCP)
Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)-Ministère de la Culture (MC)
Institut de Chimie et des Matériaux Paris-Est (ICMPE)
Institut de Chimie du CNRS (INC)-Université Paris-Est Créteil Val-de-Marne - Paris 12 (UPEC UP12)-Centre National de la Recherche Scientifique (CNRS)
European Project: 741123,CIMNAS
Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)-Ecole Nationale Supérieure de Chimie de Paris - Chimie ParisTech-PSL (ENSCP)
Université Paris sciences et lettres (PSL)-Université Paris sciences et lettres (PSL)-Ministère de la Culture (MC)
Source :
Corrosion Science, Corrosion Science, 2022, 200, pp.110233. ⟨10.1016/j.corsci.2022.110233⟩, Corrosion Science, Elsevier, 2022, 200, pp.110233. ⟨10.1016/j.corsci.2022.110233⟩
Publication Year :
2022
Publisher :
Zenodo, 2022.

Abstract

The vast composition space of the Cr-Fe-Co-Ni-Mo system was explored by massive thermodynamic calculations in order to design and characterize multi-component single-phase fcc alloys optimized in Cr and Mo content and having enhanced passivity. Adding up to 15 at.% Mo while retaining the fcc single-phase is possible, which is unprecedented. Cr is confirmed to be a prerequisite to ensure self-protection against corrosion by passivation. Adding Mo up to 10 at.% tremendously enhances the resistance to passivity breakdown in Cl--containing aggressive environment. Newly designed quinary alloys, Cr25Fe25Co5Ni40Mo5 and Cr15Fe10Co5Ni60Mo10 (at.%), show superior resistance to localized corrosion.

Details

Language :
English
ISSN :
0010938X
Database :
OpenAIRE
Journal :
Corrosion Science, Corrosion Science, 2022, 200, pp.110233. ⟨10.1016/j.corsci.2022.110233⟩, Corrosion Science, Elsevier, 2022, 200, pp.110233. ⟨10.1016/j.corsci.2022.110233⟩
Accession number :
edsair.doi.dedup.....664f0ccf9d2325a352a83ebf66f80112