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Fractional Hoppinglike Motion in Columnar Mesophases of Semiflexible Rodlike Particles

Authors :
Emilie Pouget
Paul van der Schoot
M. Paul Lettinga
Pierre Ballesta
Eric Grelet
M. Saber Naderi
Soft Matter and Biological Physics
Faculteit Technische Natuurkunde
Faculteit Technische Naturkunde
Laboratory for Acoustics and Thermal Physics [Leuven]
Catholic University of Leuven - Katholieke Universiteit Leuven (KU Leuven)
Centre de recherches Paul Pascal (CRPP)
Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)
Institut Weiche Materie (ICS-3)
Institut Weiche Materie
Instituut voor Theoretische Fysica
Universiteit Utrecht
Theoretical Physics
Afd Theoretical Physics (ITF)
Source :
Physical Review Letters, 111(3), 037801/1. American Physical Society, Physical Review Letters, 111(3):037801, 1-5. American Physical Society, Physical review letters 111(3), 037801 (2013). doi:10.1103/PhysRevLett.111.037801, Physical Review Letters, Physical Review Letters, American Physical Society, 2013, 111 (037801), pp. 1-5. ⟨10.1103/PhysRevLett.111.037801⟩
Publication Year :
2013

Abstract

International audience; We report on single-particle dynamics of strongly interacting filamentous fd virus particles in the liquidcrystalline columnar state in aqueous solution. From fluorescence microscopy, we find that rare, discrete events take place, in which individual particles engage in sudden, jumplike motion along the main rod axis. The jump length distribution is bimodal and centered at half- and full-particle lengths. Our Brownian dynamics simulations of hard semiflexible particles mimic our experiments and indicate that full-length jumps must be due to collective dynamics in which particles move in stringlike fashion in and between neighboring columns, while half jumps arise as a result of particles moving into defects. We find that the finite domain structure of the columnar phase strongly influences the observed dynamics.

Details

Language :
English
ISSN :
00319007 and 10797114
Database :
OpenAIRE
Journal :
Physical Review Letters, 111(3), 037801/1. American Physical Society, Physical Review Letters, 111(3):037801, 1-5. American Physical Society, Physical review letters 111(3), 037801 (2013). doi:10.1103/PhysRevLett.111.037801, Physical Review Letters, Physical Review Letters, American Physical Society, 2013, 111 (037801), pp. 1-5. ⟨10.1103/PhysRevLett.111.037801⟩
Accession number :
edsair.doi.dedup.....7a14512a3ebb2b5a200b89362cb0e5c4
Full Text :
https://doi.org/10.1103/PhysRevLett.111.037801