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Ultrafast dynamical response of strongly correlated oxides: role of coherent optical and acoustic oscillations

Authors :
F. Miletto Granozio
Marino Marsi
B. Mansart
Davide Boschetto
U. Scotti di Uccio
R. Malaquias
P. A. Metcalf
A. Sambri
Laboratoire de Physique des Solides (LPS)
Centre National de la Recherche Scientifique (CNRS)-Université Paris-Sud - Paris 11 (UP11)
Laboratoire d'optique appliquée (LOA)
École Nationale Supérieure de Techniques Avancées (ENSTA Paris)-École polytechnique (X)-Centre National de la Recherche Scientifique (CNRS)
CNR-INFM Coherentia
Complesso Universitario Monte S. Angelo
Dipartimento Scienze Fisiche [Napoli]
Università degli studi di Napoli Federico II
Department of Chemistry
Purdue University [West Lafayette]
B., Mansart
D., Boschetto
A., Sambri
R., Malaquia
F., Miletto Granozio
SCOTTI DI UCCIO, Umberto
P., Metcalf
M., Marsi
Source :
Journal of Modern Optics, Journal of Modern Optics, Taylor & Francis, 2010, 57 (11), pp.959-966. ⟨10.1080/09500340903541072⟩, Journal of modern optics, 57 (2010): 959. doi:10.1080/09500340903541072, info:cnr-pdr/source/autori:B. Mansart, D. Boschetto, A. Sambri, R. Malaquias, F. Miletto Granozio, U. Scotti di Uccio, P. Metcalfe, M. Marsia/titolo:Ultrafast dynamical response of strongly correlated oxides: role of coherent optical and acoustic oscillations/doi:10.1080%2F09500340903541072/rivista:Journal of modern optics (Print)/anno:2010/pagina_da:959/pagina_a:/intervallo_pagine:959/volume:57
Publication Year :
2010
Publisher :
HAL CCSD, 2010.

Abstract

International audience; We describe some general features in the transient behaviour of strongly correlated transition metal oxides, following ultrafast excitation by a femtosecond laser pulse. Our analysis is based on time-resolved reflectivity measurements on (V1-xCrx)2O3, a prototype Mott-Hubbard material, and the manganite compound (La0.67Sr0.33)MnO3, performed over a time window of several tenths of ps. We point out the contribution of coherent lattice oscillations-both optical and acoustic-to the overall signal, and show how they can depend on the crystallographic orientation of the material with respect to the laser beam wavevector and polarisation. In particular, an acoustic wave is always found to be present in our measurements, and we show that its oscillating behaviour is superposed to the average time evolution of the material, which can be instead related in different ways to its electronic properties and thermodynamic phase. All these effects are to be taken into account in any further analysis leading to the estimation of relevant physical parameters for correlated materials, and they appear to play a significant role not only for reflectivity techniques, but also in other kinds of ultrafast pump-probe experiments.

Details

Language :
English
ISSN :
09500340 and 13623044
Database :
OpenAIRE
Journal :
Journal of Modern Optics, Journal of Modern Optics, Taylor & Francis, 2010, 57 (11), pp.959-966. ⟨10.1080/09500340903541072⟩, Journal of modern optics, 57 (2010): 959. doi:10.1080/09500340903541072, info:cnr-pdr/source/autori:B. Mansart, D. Boschetto, A. Sambri, R. Malaquias, F. Miletto Granozio, U. Scotti di Uccio, P. Metcalfe, M. Marsia/titolo:Ultrafast dynamical response of strongly correlated oxides: role of coherent optical and acoustic oscillations/doi:10.1080%2F09500340903541072/rivista:Journal of modern optics (Print)/anno:2010/pagina_da:959/pagina_a:/intervallo_pagine:959/volume:57
Accession number :
edsair.doi.dedup.....7b3ff5c7723c67a14a90e8d14a5a5f68
Full Text :
https://doi.org/10.1080/09500340903541072⟩