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COVID‐19 Crisis Reduces Free Tropospheric Ozone Across the Northern Hemisphere

Authors :
Marc Allaart
Susan E. Strahan
Ryan M. Stauffer
Richard Querel
Anne M. Thompson
Nicholas B. Jones
Clare Paton-Walsh
Patrick Cullis
Tatsumi Nakano
Bryan J. Johnson
Gérard Ancellet
Thomas Blumenstock
Ankie Piters
Holger Deckelmann
Omaira García
Matthias Palm
Roeland Van Malderen
Kai-Lan Chang
Nis Jepsen
Antje Inness
M.B. Tully
Ralf Sussmann
Amelie N. Röhling
Gonzague Romanens
Dagmar Kubistin
Ana Diaz Rodriguez
Fernando Chouza
René Stübi
Owen R. Cooper
Emmanuel Mahieu
Kimberly Strong
Christian Plass-Dülmer
Jonathan Davies
Richard Engelen
Peter Oelsner
David W. Tarasick
Peter von der Gathen
Jose-Luis Hernandez
Michael Gill
Justus Notholt
Thierry Leblanc
Christian Servais
Irina Petropavlovskikh
Matthias Schneider
Norrie Lyall
Rigel Kivi
Carlos Torres
Shoma Yamanouchi
Sophie Godin-Beekmann
Bogumil Kois
James W. Hannigan
Wolfgang Steinbrecht
Andy Delcloo
Deutscher Wetterdienst [Offenbach] (DWD)
Environment and Climate Change Canada
Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung (AWI)
Danish Meteorological Institute (DMI)
Finnish Meteorological Institute (FMI)
Met Office Lerwick
Universität Bremen
Institute of Meteorology and Water Management - National Research Institute (IMGW - PIB)
Royal Netherlands Meteorological Institute (KNMI)
Irish Meteorological Service (MET ÉIREANN)
Institut Royal Météorologique de Belgique [Bruxelles] (IRM)
Institut für Meteorologie und Klimaforschung - Atmosphärische Umweltforschung (IMK-IFU)
Karlsruher Institut für Technologie (KIT)
Institut d'Astrophysique et de Géophysique [Liège]
Université de Liège
Federal Office of Meteorology and Climatology MeteoSwiss
TROPO - LATMOS
Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS)
Sorbonne Université (SU)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)
STRATO - LATMOS
University of Toronto
ESRL Global Monitoring Laboratory [Boulder] (GML)
NOAA Earth System Research Laboratory (ESRL)
National Oceanic and Atmospheric Administration (NOAA)-National Oceanic and Atmospheric Administration (NOAA)
Cooperative Institute for Research in Environmental Sciences (CIRES)
University of Colorado [Boulder]-National Oceanic and Atmospheric Administration (NOAA)
National Center for Atmospheric Research [Boulder] (NCAR)
Agencia Estatal de Meteorología (AEMet)
Meteorological Research Institute [Tsukuba] (MRI)
Japan Meteorological Agency (JMA)
Jet Propulsion Laboratory (JPL)
NASA-California Institute of Technology (CALTECH)
Institut für Meteorologie und Klimaforschung - Atmosphärische Spurengase und Fernerkundung (IMK-ASF)
Australian Bureau of Meteorology [Melbourne] (BoM)
Australian Government
University of Wollongong [Australia]
National Institute of Water and Atmospheric Research [Lauder] (NIWA)
GSFC Earth Sciences Division
NASA Goddard Space Flight Center (GSFC)
Earth Science System Interdisciplinary Center [College Park] (ESSIC)
College of Computer, Mathematical, and Natural Sciences [College Park]
University of Maryland [College Park]
University of Maryland System-University of Maryland System-University of Maryland [College Park]
University of Maryland System-University of Maryland System
European Centre for Medium-Range Weather Forecasts (ECMWF)
NOAA Chemical Sciences Laboratory (CSL)
National Oceanic and Atmospheric Administration (NOAA)
University of Wollongong
GFSC Earth Sciences Division
Kubistin, Dagmar
1 Deutscher Wetterdienst Hohenpeißenberg Germany
Plass‐Dülmer, Christian
Davies, Jonathan
2 Environment and Climate Change Canada Toronto ONT Canada
Tarasick, David W.
Gathen, Peter von der
3 Alfred Wegener Institut Helmholtz‐Zentrum für Polar‐ und Meeresforschung Potsdam Germany
Deckelmann, Holger
Jepsen, Nis
4 Danish Meteorological Institute Copenhagen Denmark
Kivi, Rigel
5 Finnish Meteorological Institute Sodankylä Finland
Lyall, Norrie
6 British Meteorological Service Lerwick UK
Palm, Matthias
7 University of Bremen Bremen Germany
Notholt, Justus
Kois, Bogumil
8 Institute of Meteorology and Water Management Legionowo Poland
Oelsner, Peter
9 Deutscher Wetterdienst Lindenberg Germany
Allaart, Marc
10 Royal Netherlands Meteorological Institute DeBilt The Netherlands
Piters, Ankie
Gill, Michael
11 Met Éireann (Irish Met. Service) Valentia Ireland
Van Malderen, Roeland
12 Royal Meteorological Institute of Belgium Uccle Belgium
Delcloo, Andy W.
Sussmann, Ralf
13 Karlsruhe Institute of Technology IMK‐IFU Garmisch‐Partenkirchen Germany
Mahieu, Emmanuel
14 Institute of Astrophysics and Geophysics University of Liège Liège Belgium
Servais, Christian
Romanens, Gonzague
15 Federal Office of Meteorology and Climatology MeteoSwiss Payerne Switzerland
Stübi, Rene
Ancellet, Gerard
16 LATMOS Sorbonne Université‐UVSQ‐CNRS/INSU Paris France
Godin‐Beekmann, Sophie
Yamanouchi, Shoma
17 University of Toronto Toronto ONT Canada
Strong, Kimberly
Johnson, Bryan
18 NOAA ESRL Global Monitoring Laboratory Boulder CO USA
Cullis, Patrick
Petropavlovskikh, Irina
Hannigan, James W.
20 National Center for Atmospheric Research Boulder CO USA
Hernandez, Jose‐Luis
21 State Meteorological Agency (AEMET) Madrid Spain
Diaz Rodriguez, Ana
Nakano, Tatsumi
22 Meteorological Research Institute Tsukuba Japan
Chouza, Fernando
23 Jet Propulsion Laboratory California Institute of Technology Table Mountain Facility Wrightwood CA USA
Leblanc, Thierry
Torres, Carlos
24 Izaña Atmospheric Research Center AEMET Tenerife Spain
Garcia, Omaira
Röhling, Amelie N.
25 Karlsruhe Institute of Technology IMK‐ASF Karlsruhe Germany
Schneider, Matthias
Blumenstock, Thomas
Tully, Matt
26 Bureau of Meteorology Melbourne Australia
Paton‐Walsh, Clare
27 Centre for Atmospheric Chemistry University of Wollongong Wollongong Australia
Jones, Nicholas
Querel, Richard
28 National Institute of Water and Atmospheric Research Lauder New Zealand
Strahan, Susan
29 NASA Goddard Space Flight Center Earth Sciences Division Greenbelt MD USA
Stauffer, Ryan M.
Thompson, Anne M.
Inness, Antje
32 European Centre for Medium‐Range Weather Forecasts Reading UK
Engelen, Richard
Chang, Kai‐Lan
19 Cooperative Institute for Research in Environmental Sciences (CIRES) University of Colorado Boulder CO USA
Cooper, Owen R.
Source :
GEOPHYSICAL RESEARCH LETTERS, Geophysical Research Letters, Geophysical Research Letters, American Geophysical Union, 2021, 48 (5), pp.e2020GL091987. ⟨10.1029/2020GL091987⟩, Geophysical Research Letters, American Geophysical Union, 2021, e2020GL091987 (in press). ⟨10.1029/2020GL091987⟩, ARCIMIS. Archivo Climatológico y Meteorológico Institucional (AEMET), Agencia Estatal de Meteorología (AEMET), Geophysical research letters, 48 (5), e2020GL091987, EPIC3Geophysical Research Letters, Wiley, 48(5), ISSN: 0094-8276
Publication Year :
2021
Publisher :
American Geophysical Union (AGU), 2021.

Abstract

Throughout spring and summer 2020, ozone stations in the northern extratropics recorded unusually low ozone in the free troposphere. From April to August, and from 1 to 8 kilometers altitude, ozone was on average 7% (≈4 nmol/mol) below the 2000–2020 climatological mean. Such low ozone, over several months, and at so many stations, has not been observed in any previous year since at least 2000. Atmospheric composition analyses from the Copernicus Atmosphere Monitoring Service and simulations from the NASA GMI model indicate that the large 2020 springtime ozone depletion in the Arctic stratosphere contributed less than one‐quarter of the observed tropospheric anomaly. The observed anomaly is consistent with recent chemistry‐climate model simulations, which assume emissions reductions similar to those caused by the COVID‐19 crisis. COVID‐19 related emissions reductions appear to be the major cause for the observed reduced free tropospheric ozone in 2020.<br />Plain Language Summary: Worldwide actions to contain the COVID‐19 virus have closed factories, grounded airplanes, and have generally reduced travel and transportation. Less fuel was burnt, and less exhaust was emitted into the atmosphere. Due to these measures, the concentration of nitrogen oxides and volatile organic compounds (VOCs) decreased in the atmosphere. These substances are important for photochemical production and destruction of ozone in the atmosphere. In clean or mildly polluted air, reducing nitrogen oxides and/or VOCs will reduce the photochemical production of ozone and result in less ozone. In heavily polluted air, in contrast, reducing nitrogen oxides can increase ozone concentrations, because less nitrogen oxide is available to destroy ozone. In this study, we use data from three types of ozone instruments, but mostly from ozonesondes on weather balloons. The sondes fly from the ground up to 30 kilometers altitude. In the first 8 km, we find significantly reduced ozone concentrations in the northern extratropics during spring and summer of 2020, less than in any other year since at least 2000. We suggest that reduced emissions due to the COVID‐19 crisis have lowered photochemical ozone production and have caused the observed ozone reductions in the troposphere.<br />Key Points: In spring and summer 2020, stations in the northern extratropics report on average 7% (4 nmol/mol) less tropospheric ozone than normal Such low tropospheric ozone, over several months, and at so many sites, has not been observed in any previous year since at least 2000 Most of the reduction in tropospheric ozone in 2020 is likely due to emissions reductions related to the COVID‐19 pandemic<br />NASA | Earth Sciences Division (NASA Earth Science Division) http://dx.doi.org/10.13039/100014573<br />Gouvernement du Canada | Natural Sciences and Engineering Research Council of Canada (NSERC) http://dx.doi.org/10.13039/501100000038<br />Australian Research Council<br />Fonds De La Recherche Scientifique ‐ FNRS (FNRS) http://dx.doi.org/10.13039/501100002661<br />Deutsche Forschungsgemeinschaft (DFG) http://dx.doi.org/10.13039/501100001659<br />Bundesministerium für Wirtschaft und Energie (BMWi) http://dx.doi.org/10.13039/501100006360

Details

ISSN :
19448007 and 00948276
Volume :
48
Database :
OpenAIRE
Journal :
Geophysical Research Letters
Accession number :
edsair.doi.dedup.....7d98cfac44905473534444dc94806757
Full Text :
https://doi.org/10.1029/2020gl091987