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High In-Plane Thermal Conductivity of Aluminum Nitride Thin Films

Authors :
Zhe Cheng
Samuel Graham
Patrick E. Hopkins
Kenny Huynh
Roisul Hasan Galib
Eric R. Hoglund
Michael E. Liao
Jeffrey L. Braun
Kamal Hussain
John A. Tomko
Shafkat Bin Hoque
Zayd C. Leseman
Mirza Elahi
David H. Olson
Mark S. Goorsky
Abdullah Mamun
Yee Rui Koh
John T. Gaskins
Zeyu Liu
James M. Howe
Asif Khan
Kiumars Aryana
Tengfei Luo
Source :
ACS Nano. 15:9588-9599
Publication Year :
2021
Publisher :
American Chemical Society (ACS), 2021.

Abstract

High thermal conductivity materials show promise for thermal mitigation and heat removal in devices. However, shrinking the length scales of these materials often leads to significant reductions in thermal conductivities, thus invalidating their applicability to functional devices. In this work, we report on high in-plane thermal conductivities of 3.05, 3.75, and 6 μm thick aluminum nitride (AlN) films measured via steady-state thermoreflectance. At room temperature, the AlN films possess an in-plane thermal conductivity of ∼260 ± 40 W m-1 K-1, one of the highest reported to date for any thin film material of equivalent thickness. At low temperatures, the in-plane thermal conductivities of the AlN films surpass even those of diamond thin films. Phonon-phonon scattering drives the in-plane thermal transport of these AlN thin films, leading to an increase in thermal conductivity as temperature decreases. This is opposite of what is observed in traditional high thermal conductivity thin films, where boundaries and defects that arise from film growth cause a thermal conductivity reduction with decreasing temperature. This study provides insight into the interplay among boundary, defect, and phonon-phonon scattering that drives the high in-plane thermal conductivity of the AlN thin films and demonstrates that these AlN films are promising materials for heat spreaders in electronic devices.

Details

ISSN :
1936086X and 19360851
Volume :
15
Database :
OpenAIRE
Journal :
ACS Nano
Accession number :
edsair.doi.dedup.....7e21e5a7223954f3a145563839a9a373
Full Text :
https://doi.org/10.1021/acsnano.0c09915