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High In-Plane Thermal Conductivity of Aluminum Nitride Thin Films
- Source :
- ACS Nano. 15:9588-9599
- Publication Year :
- 2021
- Publisher :
- American Chemical Society (ACS), 2021.
-
Abstract
- High thermal conductivity materials show promise for thermal mitigation and heat removal in devices. However, shrinking the length scales of these materials often leads to significant reductions in thermal conductivities, thus invalidating their applicability to functional devices. In this work, we report on high in-plane thermal conductivities of 3.05, 3.75, and 6 μm thick aluminum nitride (AlN) films measured via steady-state thermoreflectance. At room temperature, the AlN films possess an in-plane thermal conductivity of ∼260 ± 40 W m-1 K-1, one of the highest reported to date for any thin film material of equivalent thickness. At low temperatures, the in-plane thermal conductivities of the AlN films surpass even those of diamond thin films. Phonon-phonon scattering drives the in-plane thermal transport of these AlN thin films, leading to an increase in thermal conductivity as temperature decreases. This is opposite of what is observed in traditional high thermal conductivity thin films, where boundaries and defects that arise from film growth cause a thermal conductivity reduction with decreasing temperature. This study provides insight into the interplay among boundary, defect, and phonon-phonon scattering that drives the high in-plane thermal conductivity of the AlN thin films and demonstrates that these AlN films are promising materials for heat spreaders in electronic devices.
- Subjects :
- Work (thermodynamics)
Materials science
Scattering
General Engineering
General Physics and Astronomy
chemistry.chemical_element
02 engineering and technology
Nitride
010402 general chemistry
021001 nanoscience & nanotechnology
01 natural sciences
0104 chemical sciences
In plane
Thermal conductivity
chemistry
Aluminium
Thermal
General Materials Science
Thin film
Composite material
0210 nano-technology
Subjects
Details
- ISSN :
- 1936086X and 19360851
- Volume :
- 15
- Database :
- OpenAIRE
- Journal :
- ACS Nano
- Accession number :
- edsair.doi.dedup.....7e21e5a7223954f3a145563839a9a373
- Full Text :
- https://doi.org/10.1021/acsnano.0c09915