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Fluctuation-Dissipation Relations and Energy Landscape in an Out-of-Equilibrium Strong-Glass-Forming Liquid

Authors :
Piero Tartaglia
Antonio Scala
Francesco Sciortino
Chantal Valeriani
Source :
Scopus-Elsevier
Publication Year :
2003
Publisher :
American Physical Society (APS), 2003.

Abstract

We study the out-of-equilibrium dynamics following a temperature-jump in a model for a strong liquid, BKS-silica, and compare it with the well known case of fragile liquids. We calculate the fluctuation-dissipation relation, from which it is possible to estimate an effective temperature $T_{eff}$ associated to the slow out-of-equilibrium structural degrees of freedom. We find the striking and unexplained result that, differently from the fragile liquid cases, $T_{eff}$ is smaller than the bath temperature.

Details

ISSN :
10797114 and 00319007
Volume :
90
Database :
OpenAIRE
Journal :
Physical Review Letters
Accession number :
edsair.doi.dedup.....93ec3e34a062b757f5caeb130cadd7d5
Full Text :
https://doi.org/10.1103/physrevlett.90.115503