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Plasmons in MoS 2 studied via experimental and theoretical correlation of energy loss spectra

Authors :
Quentin M. Ramasse
Eoin Moynihan
Stefan Rost
Eoghan O'Connell
Ursel Bangert
Christoph Friedrich
IRC
Ernst Ruska-Centre, Forschungszentrum Jülich
Source :
Journal of microscopy 279(3), 256-264 (2020). doi:10.1111/jmi.12900
Publication Year :
2020
Publisher :
Wiley, 2020.

Abstract

Two dimensional materials offer a path forward for smaller and more efficient devices. Their optical and electronic properties give way to beat the limits set in place by Moore's Law. Plasmon are the collective oscillations of electrons and can confine light to dimensions much smaller than its wavelength. In this work we explore the plasmonic properties of MoS2, a representational candidate from a family of 2D materials known as transition metal dichalcogenides. High resolution electron microscopy and spectroscopy provide insights in the plasmonic properties of MoS2 down to an atomic scale. Experimental results show the relationship between plasmons and interband transitions in the electron energy loss spectrum. Density functional theory provides a theoretical support for the experimental findings and provides commentary on the fundamental underlying physics.<br />Comment: 16 pages, 5 figures, Electron Microscopy Analysis Group (EMAG) special issue

Details

ISSN :
13652818 and 00222720
Volume :
279
Database :
OpenAIRE
Journal :
Journal of Microscopy
Accession number :
edsair.doi.dedup.....95d06f85b935c325ffcaecd0a417f702
Full Text :
https://doi.org/10.1111/jmi.12900