Fractional high-harmonic combs by attosecond-precision split-spectrum pulse control

Few-cycle laser fields enable pulse-shaping control of high-order harmonic generation by time delaying variable broadband spectral sections. We report the experimental generation of fractional (noninteger) high-harmonic combs by the controlled interference of two attosecond pulse trains. Additionally the energy of the high harmonics is strongly tuned with the relative time delay. We quantify the tuning to directly result from the controlled variation of the instantaneous laser frequency at the shaped driver pulse intensity maximum.