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Seventeen years of ozone sounding at L'Aquila, Italy: evidence of mid-latitude stratospheric ozone recovery and tropospheric profile changes

Authors :
Neal Butchart
Martin Chipperfield
Slimane Bekki
Kengo Sudo
Martine Michou
Andrea Stenke
Jean-Francois Lamarque
Patrick Joeckel
Hideharu Akiyoshi
Taichu Y. Tanaka
Marco Iarlori
Marion Marchand
Giovanni Pitari
Kane A. Stone
T. Nagashima
Yousuke Yamashita
Luke D. Oman
Sandip Dhomse
Vincenzo Rizi
David Saint-Martin
Rolando R. Garcia
Guang Zeng
Simone Tilmes
Fiona M. O'Connor
Holger Tost
Irene Cionni
Robyn Schofield
Douglas E. Kinnison
David A. Plummer
Makoto Deushi
John Scinocca
Ilaria Quaglia
Olaf Morgenstern
Daniele Visioni
Eugene Rozanov
Sibley School of Mechanical and Aerospace Engineering (MAE)
Cornell University [New York]
Department of Physical and Chemical Sciences [L'Aquila] (DSFC)
Università degli Studi dell'Aquila (UNIVAQ)
Centre of Excellence CETEMPS
Agenzia Nazionale per le nuove Tecnologie, l’energia e lo sviluppo economico sostenibile (ENEA)
National Institute for Environmental Studies (NIES)
STRATO - LATMOS
Laboratoire Atmosphères, Milieux, Observations Spatiales (LATMOS)
Sorbonne Université (SU)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)
Met Office Hadley Centre for Climate Change (MOHC)
United Kingdom Met Office [Exeter]
School of Earth and Environment [Leeds] (SEE)
University of Leeds
Meteorological Research Institute [Tsukuba] (MRI)
Japan Meteorological Agency (JMA)
National Center for Atmospheric Research [Boulder] (NCAR)
DLR Institut für Physik der Atmosphäre (IPA)
Deutsches Zentrum für Luft- und Raumfahrt [Oberpfaffenhofen-Wessling] (DLR)
Centre national de recherches météorologiques (CNRM)
Institut national des sciences de l'Univers (INSU - CNRS)-Météo France-Centre National de la Recherche Scientifique (CNRS)
National Institute of Water and Atmospheric Research [Wellington] (NIWA)
NASA Goddard Space Flight Center (GSFC)
Environment and Climate Change Canada
Institute for Atmospheric and Climate Science [Zürich] (IAC)
Eidgenössische Technische Hochschule - Swiss Federal Institute of Technology [Zürich] (ETH Zürich)
School of Earth Sciences [Melbourne]
Faculty of Science [Melbourne]
University of Melbourne-University of Melbourne
Graduate School of Environmental Studies [Nagoya]
Nagoya University
Università degli Studi dell'Aquila = University of L'Aquila (UNIVAQ)
Agenzia Nazionale per le nuove Tecnologie, l’energia e lo sviluppo economico sostenibile = Italian National Agency for New Technologies, Energy and Sustainable Economic Development (ENEA)
Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Sorbonne Université (SU)-Centre National de la Recherche Scientifique (CNRS)
Institut national des sciences de l'Univers (INSU - CNRS)-Observatoire Midi-Pyrénées (OMP)
Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3)
Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3)
Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS)
Source :
Atmospheric Chemistry and Physics Discussions
Publication Year :
2020
Publisher :
HAL CCSD, 2020.

Abstract

International audience; Ozone profile measurements collected at L'Aquila (Italy, 42.4°N) during seventeen years of radio-sounding 30 (2000-2016) are presented here, with an analysis of derived trends. Model results from the SPARC-CCMI exercise are used in parallel to highlight the physical and chemical mechanisms regulating mid-latitude ozone trends. The statistically significant trends highlighted in time series at L'Aquila are those in the mid-upper stratosphere (+5.9±4.2), mid troposphere https://doi.org/10.5194/acp-2020-525 Preprint. Discussion started: 1 July 2020 c Author(s) 2020. CC BY 4.0 License. 2 (+5.9±2.4) and upper troposphere (+2.5±0.9), all in percent/decade. The upper stratospheric positive trend was already well documented in recent WMO assessments and attributed to the starting decline of stratospheric Cly and Bry and to the 35 stratospheric cooling induced by increasing well mixed greenhouse gases, thus slowing down gas-phase reactions that destroy ozone in the upper stratosphere. The ozone increase in the mid-upper troposphere is largely regulated by the increasing strength of the Brewer-Dobson circulation, which moves more ozone from the tropics to the extratropics and enhances the tropospheric influx from the lowermost stratosphere. This climate feedback mechanism on tropospheric ozone is only partially compensated by the increasing chemical ozone loss associated to higher H2O values in response to the 40 tropospheric warming. We also note that ozone trends obtained in the lower stratosphere are negative (-2.2 percent/decade), but do not result to be statistically significant in our analyses.

Details

Language :
English
ISSN :
16807367 and 16807375
Database :
OpenAIRE
Journal :
Atmospheric Chemistry and Physics Discussions
Accession number :
edsair.doi.dedup.....9ec8239db4c94133ce9ac4cb4e8c6b07