Closed-Loop Recycling of Both Resin and Fiber from High-Performance Thermoset Epoxy/Carbon Fiber Composites

Currently, only 5% of thermoset carbon fiber reinforced polymer composites (CFRPs) are recycled into lower-value secondary products. Highly efficient closed-loop recycling of both thermoset resin and carbon fiber is a major challenge. Here, we report a sustainable approach for the closed-loop recycling of the resin and fiber from CFRPs. Thiol-functionalized carbon fiber (TCF) obtained by functionalization with a thiol-ended hyperbranched polymer, and then an epoxy-ended degradable hyperbranched polymer (HT