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Highly efficient near-infrared quantum cutting in Ce3+/Yb3+ co-doped chalcohalide glasses

Authors :
Hongli Ma
Jean-Luc Adam
Bing Gao
Qiqi Yan
Xianghua Zhang
Yu Tong
Jing Ren
Guorong Chen
Key Laboratory for Ultrafine Materials of Ministry of Education
East China University of Science and Technology
Institut des Sciences Chimiques de Rennes (ISCR)
Université de Rennes (UR)-Institut National des Sciences Appliquées - Rennes (INSA Rennes)
Institut National des Sciences Appliquées (INSA)-Institut National des Sciences Appliquées (INSA)-Ecole Nationale Supérieure de Chimie de Rennes (ENSCR)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)
Shanghai Leading Academic Discipline Project (No. B502), Shanghai Key Laboratory Project (08DZ2230500)
Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC)-Université de Rennes 1 (UR1)
Université de Rennes (UNIV-RENNES)-Université de Rennes (UNIV-RENNES)-Ecole Nationale Supérieure de Chimie de Rennes (ENSCR)-Institut National des Sciences Appliquées - Rennes (INSA Rennes)
Institut National des Sciences Appliquées (INSA)-Université de Rennes (UNIV-RENNES)-Institut National des Sciences Appliquées (INSA)
Source :
Journal of Luminescence, Journal of Luminescence, 2013, 143, pp.181-184. ⟨10.1016/j.jlumin.2013.04.015⟩, Journal of Luminescence, Elsevier, 2013, 143, pp.181-184. ⟨10.1016/j.jlumin.2013.04.015⟩
Publication Year :
2013
Publisher :
HAL CCSD, 2013.

Abstract

International audience; Near-infrared (NIR) quantum cutting involving the emission of two NIR photons for each visible photon absorbed is realized from Ce3+/Yb3+ codoped chalcohalide glasses. Excitation, emission and decay spectra are measured to prove the occurrence of energy transfer (ET) from Ce3+ to Yb3+. The maximum ET efficiency obtained is as high as 82%, and the possible mechanism of ET is discussed. The directly measured and calculated quantum yield (QY) of the Yb3+ emission upon the excitation of 5d level of Ce3+ is up to 119%.

Details

Language :
English
ISSN :
00222313 and 18727883
Database :
OpenAIRE
Journal :
Journal of Luminescence, Journal of Luminescence, 2013, 143, pp.181-184. ⟨10.1016/j.jlumin.2013.04.015⟩, Journal of Luminescence, Elsevier, 2013, 143, pp.181-184. ⟨10.1016/j.jlumin.2013.04.015⟩
Accession number :
edsair.doi.dedup.....a919eac2f5d7e582af916658295b9ad5