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Dynamics of liquids in the large-dimensional limit
- Source :
- Physical Review E. 104
- Publication Year :
- 2021
- Publisher :
- American Physical Society (APS), 2021.
-
Abstract
- In this paper we analytically derive the exact closed dynamical equations for a liquid with short-ranged interactions in large spatial dimensions using the same statistical mechanics tools employed to analyze Brownian motion. Our derivation greatly simplifies the original path-integral-based route to these equations and provides insight into the physical features associated with high-dimensional liquids and glass formation. Most importantly, our construction provides a route to the exact dynamical analysis of important related dynamical problems, as well as a means to devise cluster generalizations of the exact solution in infinite dimensions. This latter fact opens the door to the construction of increasingly accurate theories of vitrification in three-dimensional liquids.
Details
- ISSN :
- 24700053 and 24700045
- Volume :
- 104
- Database :
- OpenAIRE
- Journal :
- Physical Review E
- Accession number :
- edsair.doi.dedup.....b0c0e9c352c78f367c8e851bd186c656
- Full Text :
- https://doi.org/10.1103/physreve.104.054606