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Autocatalytic Reaction Fronts Inside a Porous Medium of Glass Spheres

Authors :
Severine Atis
Sandeep Saha
Harold Auradou
Dominique Salin
Laurent Talon
Fluides, automatique, systèmes thermiques (FAST)
Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)
Source :
Physical Review Letters, Physical Review Letters, American Physical Society, 2013, 110 (14), pp.013102. ⟨10.1103/PhysRevLett.110.148301⟩
Publication Year :
2013
Publisher :
HAL CCSD, 2013.

Abstract

We analyze experimentally chemical waves propagation in the disordered flow field of a porous medium. The reaction fronts travel at a constant velocity which drastically depends on the mean flow direction and rate. The fronts may propagate either downstream and upstream but, surprisingly, they remain static over a range of flow rate values. Resulting from the competition between the chemical reaction and the disordered flow field, these frozen fronts display a particular sawtooth shape. The frozen regime is likely to be associated with front pinning in low velocity zones, the number of which varies with the ratio of the mean flow and the chemical front velocities. PACS numbers

Details

Language :
English
ISSN :
00319007 and 10797114
Database :
OpenAIRE
Journal :
Physical Review Letters, Physical Review Letters, American Physical Society, 2013, 110 (14), pp.013102. ⟨10.1103/PhysRevLett.110.148301⟩
Accession number :
edsair.doi.dedup.....b750320072be2658f7d843ea435a7c0b
Full Text :
https://doi.org/10.1103/PhysRevLett.110.148301⟩