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Asymmetric Chiral Ligand-Directed Alkene Dioxygenation

Authors :
Sharon R. Neufeldt
Melanie S. Sanford
Source :
Organic Letters. 15:46-49
Publication Year :
2012
Publisher :
American Chemical Society (ACS), 2012.

Abstract

A Pd-catalyzed asymmetric alkene 1,2-dioxygenation reaction is described. The diastereoselectivity of the reaction is controlled by tethering a chiral oxime ether directing group to the alkene substrate. The best selectivities are obtained with 8-substituted menthone-derived oxime ether auxiliaries.

Details

ISSN :
15237052 and 15237060
Volume :
15
Database :
OpenAIRE
Journal :
Organic Letters
Accession number :
edsair.doi.dedup.....badff4ad7c05e2f4ed3a87006dbf3063
Full Text :
https://doi.org/10.1021/ol303003g