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Dynamic complexation of copper(I) chloride by carbene-stabilized disilicon

Authors :
Gregory H. Robinson
Mingwei Chen
Paul von Ragué Schleyer
Nichole A. Schwartz
Pingrong Wei
Yaoming Xie
Yu-Zhong Wang
Henry F. Schaefer
Robert J. Gilliard
Source :
Chemistry (Weinheim an der Bergstrasse, Germany). 20(30)
Publication Year :
2014

Abstract

Reaction of N-heterocyclic-carbene (NHC)-stabilized disilicon (1) with CuCl gave a carbene-stabilized disilicon-copper(I) chloride complex (2). The nature of the structure and bonding in 2 has been investigated by crystallographic, spectroscopic, and computational methods. The dynamic complexation behavior of 2 was experimentally explored by variable-temperature NMR analysis.

Details

ISSN :
15213765
Volume :
20
Issue :
30
Database :
OpenAIRE
Journal :
Chemistry (Weinheim an der Bergstrasse, Germany)
Accession number :
edsair.doi.dedup.....c38fdd3e6444eb523077b927cf4b7f1d