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Continental and Ecoregion‐Specific Drivers of Atmospheric NO 2 and NH 3 Seasonality Over Africa Revealed by Satellite Observations
- Source :
- Global Biogeochemical Cycles, Global Biogeochemical Cycles, 2021, 35, ⟨10.1029/2020GB006916⟩
- Publication Year :
- 2021
- Publisher :
- American Geophysical Union (AGU), 2021.
-
Abstract
- International audience; Ammonia (NH3) and nitrogen oxides (NOx: nitrogen dioxide [NO2] + nitric oxide [NO]) play important roles in atmospheric chemistry. Throughout most of Africa, emissions of these gases are predominantly from soils and biomass burning. Here we use observations of tropospheric NO2 vertical column densities (VCDs) from the Ozone Monitoring Instrument from 2005 through 2017 and atmospheric NH3 VCDs from the Infrared Atmospheric Sounding Interferometer from 2008 through 2017 to evaluate seasonal variation of NO2 and NH3 VCDs across Africa and in seven African ecoregions. In regions where mean annual precipitation (MAP) is under 500 mm yr−1, we find that NO2 and NH3 VCDs are positively related to monthly precipitation, and where MAP is between 500 and 1,750 mm yr−1 or higher, NO2 VCDs are negatively related to monthly precipitation. In dry ecoregions, temperature and precipitation were important predictors of NH3 and NO2 VCDs, likely related to variation in soil emissions. In mesic ecoregions, monthly NO2 VCDs were strongly related to burned area, suggesting that biomass burning drives seasonality. NH3 VCDs in mesic ecoregions were positively related to both monthly temperature and monthly carbon monoxide (CO) VCDs, suggesting that a mixture of soil and biomass burning emissions influenced NH3 seasonality. In northern mesic ecoregions, monthly temperature explained most of the variance in monthly NH3 VCDs, suggesting that soil sources, including animal excreta, determined NH3 seasonality. In southern mesic ecoregions, monthly CO VCDs explained more variation in NH3 VCDs than temperature, suggesting that biomass burning may have greater influence over NH3 seasonality.
- Subjects :
- Atmospheric Science
Global and Planetary Change
Air pollution
[SDU.STU]Sciences of the Universe [physics]/Earth Sciences
Seasonality
medicine.disease_cause
Atmospheric sciences
medicine.disease
Trace gas
remote sensing
nitrogen cycling
Ecoregion
trace gases
[SDU]Sciences of the Universe [physics]
Remote sensing (archaeology)
troposphere: composition and chemistry
Soil water
medicine
Environmental Chemistry
Environmental science
Satellite
biosphere/atmosphere interactions
Nitrogen cycle
General Environmental Science
Subjects
Details
- ISSN :
- 19449224 and 08866236
- Volume :
- 35
- Database :
- OpenAIRE
- Journal :
- Global Biogeochemical Cycles
- Accession number :
- edsair.doi.dedup.....c72a964f9fbfd930fd33fd5eb3244886
- Full Text :
- https://doi.org/10.1029/2020gb006916