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Imaging orbital-selective quasiparticles in the Hund's metal state of FeSe

Authors :
Brian M. Andersen
Peter O. Sprau
Paul C. Canfield
J. C. Séamus Davis
Andreas Kreisel
Andrey Kostin
Anna E. Böhmer
Peter Hirschfeld
Yi Xue Chong
Source :
Nature materials. 17(10)
Publication Year :
2018

Abstract

Strong electronic correlations, emerging from the parent Mott insulator phase, are key to copper-based high temperature superconductivity (HTS). By contrast, the parent phase of iron-based HTS is never a correlated insulator. But this distinction may be deceptive because Fe has five active d-orbitals while Cu has only one. In theory, such orbital multiplicity can generate a Hund's Metal state, in which alignment of the Fe spins suppresses inter-orbital fluctuations producing orbitally selective strong correlations. The spectral weights $Z_m$ of quasiparticles associated with different Fe orbitals m should then be radically different. Here we use quasiparticle scattering interference resolved by orbital content to explore these predictions in FeSe. Signatures of strong, orbitally selective differences of quasiparticle $Z_m$ appear on all detectable bands over a wide energy range. Further, the quasiparticle interference amplitudes reveal that $Z_{xy}<br />Comment: for movie M1, see http://www.physik.uni-leipzig.de/~kreisel/osqp/M1.mp4, for movie M2, see http://www.physik.uni-leipzig.de/~kreisel/osqp/M2.mp4, for movie M3, see http://www.physik.uni-leipzig.de/~kreisel/osqp/M3.mp4, for movie M4, see http://www.physik.uni-leipzig.de/~kreisel/osqp/M4.mp4, for movie M5, see http://www.physik.uni-leipzig.de/~kreisel/osqp/M5.mp4

Details

ISSN :
14764660
Volume :
17
Issue :
10
Database :
OpenAIRE
Journal :
Nature materials
Accession number :
edsair.doi.dedup.....cb807655fce3b8f80bac1601a2bbad0c