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Palladium-Catalyzed Regioselective Arylalkenylation of Ynamides

Authors :
Rajeshwer Vanjari
Shubham Dutta
Shengwen Yang
Vincent Gandon
Akhila K. Sahoo
Source :
Organic Letters. 24:1524-1529
Publication Year :
2022
Publisher :
American Chemical Society (ACS), 2022.

Abstract

A cationic palladium-catalyzed arylalkenylation of ynamides is presented. The putative keteniminium arylpalladium intermediate likely dictates the regioselective carbopalladation of the ynamide to form a vinylpalladium species. The capture of this complex by the olefin yields linear conjugated β-alkenyl aminodienes (especially with

Details

ISSN :
15237052 and 15237060
Volume :
24
Database :
OpenAIRE
Journal :
Organic Letters
Accession number :
edsair.doi.dedup.....e0d728297d4537e000af69d69765e75a