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Stream pollution concentration in riffle geomorphic units (Yzeron basin, France)

Authors :
Claire Bordes
Philippe Namour
Guillaume Fantino
Bertrand Moulin
Laurent Schmitt
David Eschbach
Pascal Breil
Milieux aquatiques, écologie et pollutions (UR MALY)
Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)
River Monitoring & Management - Suivi et gestion des rivières (2014-2016)
Institut des Sciences Analytiques (ISA)
Institut de Chimie du CNRS (INC)-Université Claude Bernard Lyon 1 (UCBL)
Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC)-Université Claude Bernard Lyon 1 (UCBL)
Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS)
Laboratoire Image, Ville, Environnement (LIVE)
Université de Strasbourg (UNISTRA)-Centre National de la Recherche Scientifique (CNRS)
AEMGEO
Chemometrics and Theoretical Chemistry - Chimiométrie et chimie théorique
Hydrologie-Hydraulique (UR HHLY)
The authors thank the French National Research Agency (INVASION ANR-08-CESA-022 and EPEC ANR-10-ECOT-007), the Field Observatory in Urban Water Management (OTHU - www.othu.org/ - FED 4161), the Greater Lyon, the Rhone-Mediterranean & Corsica Water Agency, and the Rhone-Alpes Region for their scientific and financial support.
ANR-08-CESA-0022,INVASION,les contaminants microbiens introduits lors dévènements pluieux dans les milieu péri-urbain: conséquences écologiques et dangers pour la santé(2008)
ANR-10-ECOT-0007,EPEC(2010)
River Monitoring & Management - Suivi et gestion des rivières
Centre National de la Recherche Scientifique (CNRS)-Université de Lyon-Université Claude Bernard Lyon 1 (UCBL)
Université de Lyon-École normale supérieure - Lyon (ENS Lyon)-Centre National de la Recherche Scientifique (CNRS)-Université de Lyon-Université Claude Bernard Lyon 1 (UCBL)
Université de Lyon-École normale supérieure - Lyon (ENS Lyon)
École normale supérieure - Lyon (ENS Lyon)-Université Claude Bernard Lyon 1 (UCBL)
Université de Lyon-Université de Lyon-Centre National de la Recherche Scientifique (CNRS)-École normale supérieure - Lyon (ENS Lyon)-Université Claude Bernard Lyon 1 (UCBL)
Source :
Science of the Total Environment, Science of the Total Environment, Elsevier, 2015, 532, 532, pp.80-90. ⟨10.1016/j.scitotenv.2015.05.057⟩, Science of the Total Environment, Elsevier, 2015, 532, pp.80-90. ⟨10.1016/j.scitotenv.2015.05.057⟩
Publication Year :
2015
Publisher :
Elsevier BV, 2015.

Abstract

International audience; In urbanized areas, small streams can be greatly damaged by urban inflows and combined sewer overflows. These polluted inputs can be several times higher than the natural stream flow over short time periods. Sound knowledge of the spatial distribution of the discharged pollutants in sediments is therefore crucial for designing monitoring strategies and suitable remediation operations. This field study combines geomorphic characterization, hydraulic conductivity measurement and pollutant assays in sediments of a small suburban river. The study site was divided up into geomorphic units: riffles, pools and runs. The last two were grouped into one class named "pool-runs" owing to their closely similar open channel flow hydraulics. Benthic and hyporheic sediments were sampled at 2 m intervals. Conventional particulate pollutants (Cr, Pb, N-org, P-tot& C-org) were assayed in samples. The main result was: pollutants were not randomly distributed in the stream sediments, but their location showed clear concentration differences by geomorphic units, with preferential accumulation in the hyporheic zones of riffle units and a lesser one in the hyporheic zones of pools. A decrease in hydraulic conductivity was significantly correlated with an increase in pollutant concentration. This occurred mainly at the transition between riffles and pool units. The down-welling water fluxes in the sediment calculated using Darcy's formula reflect this slowdown. Our findings highlight the need to take into account the geomorphological and hydrological functioning of a stream to accurately locate the biogeochemical hotspots to be treated and thereby develop more relevant monitoring and remediation methodologies.

Details

ISSN :
00489697 and 18791026
Volume :
532
Database :
OpenAIRE
Journal :
Science of The Total Environment
Accession number :
edsair.doi.dedup.....ea284266deeee86560fa6c62f8b59412