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Design of cyclometallated 5-π-delocalized donor-1,3-di(2-pyridyl)benzene platinum(II) complexes with second-order nonlinear optical properties

Authors :
Véronique Guerchais
Simona Fantacci
Julien Boixel
Dominique Roberto
Alessia Colombo
Stefania Righetto
Eleonora Garoni
Claudia Dragonetti
Nicolò Baggi
Università degli Studi di Milano = University of Milan (UNIMI)
Institut des Sciences Chimiques de Rennes (ISCR)
Université de Rennes (UR)-Institut National des Sciences Appliquées - Rennes (INSA Rennes)
Institut National des Sciences Appliquées (INSA)-Institut National des Sciences Appliquées (INSA)-Ecole Nationale Supérieure de Chimie de Rennes (ENSCR)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)
Istituto di Scienze e Tecnologie Molecolari (ISTM)
National Research Council of Italy | Consiglio Nazionale delle Ricerche (CNR)
CNR, Center for Neuroscience Research
CNRS, Centre National de la Recherche Scientifique
MIUR, Ministero dell’Istruzione, dell’Università e della Ricerca
Università degli Studi di Milano [Milano] (UNIMI)
Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC)-Université de Rennes 1 (UR1)
Université de Rennes (UNIV-RENNES)-Université de Rennes (UNIV-RENNES)-Ecole Nationale Supérieure de Chimie de Rennes (ENSCR)-Institut National des Sciences Appliquées - Rennes (INSA Rennes)
Institut National des Sciences Appliquées (INSA)-Université de Rennes (UNIV-RENNES)-Institut National des Sciences Appliquées (INSA)
Consiglio Nazionale delle Ricerche [Roma] (CNR)
Source :
Polyhedron, Polyhedron, 2018, 140, pp.74-77. ⟨10.1016/j.poly.2017.11.051⟩, Polyhedron 140 (2018): 74–77. doi:10.1016/j.poly.2017.11.051, info:cnr-pdr/source/autori:Baggi, Nicolo; Garoni, Eleonora; Colombo, Alessia; Dragonetti, Claudia; Righetto, Stefania; Roberto, Dominique; Boixel, Julien; Guerchais, Veronique; Fantacci, Simona/titolo:Design of cyclometallated 5-pi-delocalized donor-1,3-di(2-pyridyl)benzene platinum(II) complexes with second-order nonlinear optical properties/doi:10.1016%2Fj.poly.2017.11.051/rivista:Polyhedron/anno:2018/pagina_da:74/pagina_a:77/intervallo_pagine:74–77/volume:140, Polyhedron, Elsevier, 2018, 140, pp.74-77. ⟨10.1016/j.poly.2017.11.051⟩
Publication Year :
2018
Publisher :
Elsevier BV, 2018.

Abstract

The effect on the second-order nonlinear optical properties of the nature of the pi-delocalized moiety in the position 5 of a 1,3-di(2-pyridyl)benzene cyclometallated to a platinum(II) center was investigated. The influence of the substitution of a double bond with a triple bond as bridge between a triphenylamino group and the cyclometallated phenyl ring was studied and turned out to be negligible. Remarkably, the novel easily-prepared platinum(II) complex with a cyclometallated 5-styryl-1,3-di(2-pyridyl)benzene is characterized by a good second-order NLO response, as determined in solution by the EFISH technique; it is a good candidate for application in photonics. (C) 2017 Elsevier Ltd. All rights reserved.

Details

ISSN :
02775387
Volume :
140
Database :
OpenAIRE
Journal :
Polyhedron
Accession number :
edsair.doi.dedup.....edc6c0ee943fc7f21f217070ecd5c504