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Charge and Orbital Order in Half-Doped Manganites

Authors :
Daniel I. Khomskii
Giniyat Khaliullin
J.E. van den Brink
Computational Materials Science
Faculty of Science and Engineering
Source :
Physical review letters, 83(24), 5118-5121. American Physical Society, Physical Review Letters, 83(24), 5118-5121. AMER PHYSICAL SOC
Publication Year :
1999

Abstract

An explanation is given for the charge order, orbital order and insulating state observed in half-doped manganese oxides, such as Nd$_{1/2}$Sr$_{1/2}$MnO$_{3}$. The competition between the kinetic energy of the electrons and the magnetic exchange energy drives the formation of effectively one-dimensional ferromagnetic zig-zag chains. Due to a topological phase factor in the hopping, the chains are intrinsically insulating and orbital-ordered. Most surprisingly, the strong Coulomb interaction between electrons on the same Mn-ion leads to the experimentally observed charge ordering. For doping less than 1/2 the system is unstable towards phase separation into a ferromagnetic metallic and charge-ordered insulating phase.<br />To appear in Phys. Rev. Lett., 4 pages, 4 figures

Details

ISSN :
00319007
Database :
OpenAIRE
Journal :
Physical review letters, 83(24), 5118-5121. American Physical Society, Physical Review Letters, 83(24), 5118-5121. AMER PHYSICAL SOC
Accession number :
edsair.doi.dedup.....efba7a8c2012a61fd7be3165f7beee86