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Ubiquity of amplitude-modulated magnetic ordering in the $H − T$ phase diagram of the frustrated non-Fermi-liquid YbAgGe

Authors :
Garry J. McIntyre
Ch. Rüegg
D. F. McMorrow
Oksana Zaharko
C. B. Larsen
B. Fåk
Eric Ressouche
S.L. Bud'ko
D. G. Mazzone
Emmanuel Canévet
P. C. Canfield
Laboratory for Neutron Scattering and Imaging [Paul Scherrer Institute] (LNS)
Paul Scherrer Institute (PSI)
Department of Quantum Matter Physics [Geneva] (DQMP)
University of Geneva [Switzerland]
London Centre for Nanotechnology
University College of London [London] (UCL)
Institut Laue-Langevin (ILL)
ILL
Magnétisme et Diffusion Neutronique (MDN )
Modélisation et Exploration des Matériaux (MEM)
Institut de Recherche Interdisciplinaire de Grenoble (IRIG)
Direction de Recherche Fondamentale (CEA) (DRF (CEA))
Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Direction de Recherche Fondamentale (CEA) (DRF (CEA))
Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Grenoble Alpes (UGA)-Institut de Recherche Interdisciplinaire de Grenoble (IRIG)
Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Grenoble Alpes (UGA)
Ames Laboratory [Ames, USA]
Iowa State University (ISU)-U.S. Department of Energy [Washington] (DOE)
the Swiss National Science Foundation (Grant No. 200020-182536)
Université de Genève = University of Geneva (UNIGE)
Source :
Physical Review B, Physical Review B, American Physical Society, 2021, 104, pp.054424. ⟨10.1103/PhysRevB.104.054424⟩, Physical Review B, 2021, 104, pp.054424. ⟨10.1103/PhysRevB.104.054424⟩
Publication Year :
2021
Publisher :
HAL CCSD, 2021.

Abstract

International audience; YbAgGe contains a magnetic geometrically frustrated kagome-like lattice that also features significant local single-ion anisotropy. The electronic state is established by hybridization of $4f$ and conduction electrons leading to heavy electronic masses. The competition between these various interactions leads to nontrivial behavior under external magnetic field, including a sequence of magnetic phase transitions, non-Fermi-liquid states, and possibly a quantum critical point. We present a series of neutron diffraction experiments performed in the mK temperature range and under magnetic fields up to 8 T in the hexagonal plane, revealing the microscopic nature of the first four subsequent magnetic states of this phase diagram. The magnetic phases are associated with the propagation vectors $k_1$ = (${1\over 3}$ 0 ${1\over 3}$) for $H$ < 2 T, $k_2$ = (0 0 0.32) for 2 T < $H$ < 3 T, $k_1$ = (${1\over 3}$ 0 ${1\over 3}$) for 3 T < $H$ < 4.5 T, and $k_3$ = (0.195 0.195 0.38) for 4.5 T < $H$ < 7 T. Our structural refinements reveal a strong modulation of the magnetic moment amplitude in all phases. We observe that the ordered moments of the three magnetically different Yb sites become increasingly different in field, which complies with the principle local anisotropy directions relative to the field direction. While the ordered moments are aligned predominantly in the hexagonal plane, we also find a significant out-of-plane component and a ferromagnetic contribution above 2 T. We discuss possible scenarios that may evolve around the phase boundary at 4.5 T, which is associated with putative quantum criticality as identified by various bulk probes. We propose further steps that are required to better understand the microscopic interactions in this material.

Details

Language :
English
ISSN :
24699950 and 24699969
Database :
OpenAIRE
Journal :
Physical Review B, Physical Review B, American Physical Society, 2021, 104, pp.054424. ⟨10.1103/PhysRevB.104.054424⟩, Physical Review B, 2021, 104, pp.054424. ⟨10.1103/PhysRevB.104.054424⟩
Accession number :
edsair.doi.dedup.....f41f2cadd8730535370fc2c2f8563acf