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Machine learning guided microwave-assisted quantum dot synthesis and an indication of residual H

Authors :
Quan, Xu
Yaoyao, Tang
Peide, Zhu
Weiye, Zhang
Yuqi, Zhang
Oliver Sanchez, Solis
Travis Shihao, Hu
Juncheng, Wang
Source :
Nanoscale. 14(37)
Publication Year :
2022

Abstract

The current preparation methods of carbon quantum dots (CDs) involve many reaction parameters, which leads to many possibilities in the synthesis processes and high uncertainty of the resultant production performance. Recently, machine learning (ML) methods have shown great potential in correlating the selected features in many applications, which can help understand the relevant structure-function relationships of CDs and discover better synthesis recipes as well. In this work, we employ the ML approach to guide the blue CD synthesis in microwave systems. After optimizing the synthesis parameters and conditions, the quantum yield (QY) increases to about 200% higher than the average value of the prepared samples without ML guidance. The obtained CDs are applied as fluorescent probes to monitor hydrogen peroxide (H

Details

ISSN :
20403372
Volume :
14
Issue :
37
Database :
OpenAIRE
Journal :
Nanoscale
Accession number :
edsair.pmid..........8eebc28d520623b448b1f6dcc7bfdf3b