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Signatures of Dynamical Heterogeneity in the Structure of Glassy Free-energy Minima

Authors :
Chaudhuri, Pinaki
Karmakar, Smarajit
Dasgupta, Chandan
Source :
Phys. Rev. Lett. 100, 125701 (2008)
Publication Year :
2007

Abstract

From numerical minimization of a model free energy functional for a system of hard spheres, we show that the width of the local peaks of the time-averaged density field at a glassy free-energy minimum exhibits large spatial variation, similar to that of the ``local Debye-Waller factor'' in simulations of dynamical heterogeneity. Molecular dynamics simulations starting from a particle configuration generated from the density distribution at a glassy free-energy minimum show similar spatial heterogeneity in the degree of localization, implying a direct connection between dynamical heterogeneity and the structure of glassy free energy minima.<br />Comment: 5 pages, 5 figures

Details

Database :
arXiv
Journal :
Phys. Rev. Lett. 100, 125701 (2008)
Publication Type :
Report
Accession number :
edsarx.0711.4269
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevLett.100.125701