Start Over

Resonant elastic soft x-ray scattering in oxygen-ordered YBa_2Cu_3O_{6+delta}

Authors :: Hawthorn, D. G.
Shen, K. M.
Geck, J.
Peets, D. C.
Wadati, H.
Okamoto, J.
Huang, S. -W.
Huang, D. J.
Lin, H. -J.
Denlinger, J. D.
Liang, Ruixing
Bonn, D. A.
Hardy, W. N.
Sawatzky, G. A.
Source :: Phys. Rev. B 84, 075125 (2011)
Publication Year :: 2011
Abstract: Static charge-density wave (CDW) and spin-density wave (SDW) order has been convincingly observed in La-based cuprates for some time. However, more recently it has been suggested by quantum oscillation, transport and thermodynamic measurements that density wave order is generic to underdoped cuprates and plays a significant role in YBa_2Cu_3O_{6+delta} (YBCO). We use resonant soft x-ray scattering at the Cu L and O K edges to search for evidence of density wave order in Ortho-II and Ortho-VIII oxygen-ordered YBCO. We report a null result -- no evidence for static CDW order -- in both Ortho-II and Ortho-VIII ordered YBCO. While this does not rule out static CDW order in the CuO_2 planes of YBCO, these measurements place limits on the parameter space (temperature, magnetic field, scattering vector) in which static CDW order may exist. In addition, we present a detailed analysis of the energy and polarization dependence of the Ortho-II superstructure Bragg reflection [0.5 0 0] at the Cu L edge. The intensity of this peak, which is due to the valence modulations of Cu in the chain layer, is compared with calculations using atomic scattering form factors deduced from x-ray absorption measurements. The calculated energy and polarization dependence of the scattering intensity is shown to agree very well with the measurement, validating the approach and providing a framework for analyzing future resonant soft x-ray scattering measurements.<br />Comment: 11 pages, 9 figures