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Ultrafast Energy Transfer Between Molecular Assemblies and Surface Plasmons in the Strong Coupling Regime
- Publication Year :
- 2013
-
Abstract
- The nonlinear optical dynamics of nano-materials comprised of plasmons interacting with quantum emitters is investigated by a self-consistent model based on the coupled Maxwell-Liouville-von Neumann equations. It is shown that ultra-short resonant laser pulses significantly modify the optical properties of such hybrid systems. It is further demonstrated that the energy transfer between interacting molecules and plasmons occurs on a femtosecond time scale and can be controlled with both material and laser parameters.<br />Comment: 15 pages, 9 figures, submitted to ACS Nano
- Subjects :
- Condensed Matter - Mesoscale and Nanoscale Physics
Physics - Optics
Subjects
Details
- Database :
- arXiv
- Publication Type :
- Report
- Accession number :
- edsarx.1308.5012
- Document Type :
- Working Paper
- Full Text :
- https://doi.org/10.1021/nn4054528