Quantum-enhanced tomography of unitary processes

A fundamental task in photonics is to characterise an unknown optical process, defined by properties such as birefringence, spectral response, thickness and flatness. Amongst many ways to achieve this, single-photon probes can be used in a method called quantum process tomography (QPT). Furthermore, QPT is an essential method in determining how a process acts on quantum mechanical states. For example for quantum technology, QPT is used to characterise multi-qubit processors and quantum communication channels; across quantum physics QPT of some form is often the first experimental investigation of a new physical process, as shown in the recent research into coherent transport in biological mechanisms. However, the precision of QPT is limited by the fact that measurements with single-particle probes are subject to unavoidable shot noise---this holds for both single photon and laser probes. In situations where measurement resources are limited, for example, where the process is rapidly changing or the time bandwidth is constrained, it becomes essential to overcome this precision limit. Here we devise and demonstrate a scheme for tomography which exploits non-classical input states and quantum interferences; unlike previous QPT methods our scheme capitalises upon the possibility to use simultaneously multiple photons per mode. The efficiency---quantified by precision per photon used---scales with larger photon number input states. Our demonstration uses four-photon states and our results show a substantial reduction of statistical fluctuations compared to traditional QPT methods---in the ideal case one four-photon probe state yields the same amount of statistical information as twelve single probe photons.