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Effect of Chemical Pressure on High Temperature Ferrimagnetic Double Perovskites Sr2CrOsO6 and Ca2CrOsO6

Authors :
Morrow, Ryan
Soliz, Jennifer R.
Hauser, Adam J.
Gallagher, James C.
Susner, Michael A.
Sumption, Michael D.
Aczel, Adam A.
Yan, Jiaqiang
Yang, Fengyuan
Woodward, Patrick M.
Source :
J Solid State Chem 238, 46-52 (2016)
Publication Year :
2015

Abstract

The ordered double perovskites Sr2CrOsO6 and Ca2CrOsO6 have been synthesized and characterized with neutron powder diffraction, electrical transport measurements, and high field magnetization experiments. Sr2CrOsO6 and Ca2CrOsO6 crystallize with R-3 and P21/n space group symmetry, respectively. Both materials are found to be ferrimagnetic insulators with saturation magnetizations near 0.2 {\mu}B. Sr2CrOsO6 orders at 660 K, showing non-monotonic magnetization temperature dependence, while Ca2CrOsO6 orders at 490 K and does not show non-monotonic behavior. Evidence for a theoretically predicted canted magnetic structure in Sr2CrOsO6 is sought and not found.<br />Comment: 18 pages and 8 figures

Details

Database :
arXiv
Journal :
J Solid State Chem 238, 46-52 (2016)
Publication Type :
Report
Accession number :
edsarx.1509.00901
Document Type :
Working Paper
Full Text :
https://doi.org/10.1016/j.jssc.2016.02.025