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Multilayer Silicene: a clear evidence

Authors :
De Padova, Paola
Generosi, Amanda
Paci, Barbara
Ottaviani, Carlo
Quaresima, Claudio
Olivieri, Bruno
Salomon, Eric
Angot, Thierry
Lay, Guy Le
Publication Year :
2016

Abstract

One year after the publication of the seminal paper on monolayer 3 by 3 reconstructed silicene grown on a silver (111) substrate, evidence of the synthesis of epitaxial root3 by root3 reconstructed multilayer silicene hosting Dirac fermions was presented. Although a general consensus was immediately reached in the former case, in the latter one, the mere existence of multilayer silicene was questioned and strongly debated. Here, we demonstrate by means of a comprehensive x-ray crystallographic study, that multilayer silicene is effectively realized upon growth at rather low growth temperatures (~200{\deg}C), while, instead, 3D growth of silicon crystallites takes place at higher temperatures, (~300{\deg}C). This transition to bulk like silicon perfectly explains the various data presented and discussed in the literature and solves their conflicting interpretations.

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.1606.05919
Document Type :
Working Paper