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Inversion of Strong Field Photoelectron Spectra for Molecular Orbital Imaging

Authors :
Puthumpally-Joseph, R.
Viau-Trudel, J.
Peters, M.
Nguyen-Dang, T. T.
Atabek, O.
Charron, E.
Source :
Phys. Rev. A 94, 023421 (2016)
Publication Year :
2016

Abstract

Imaging structures at the molecular level is a fast developing interdisciplinary research field that spans across the boundaries of physics and chemistry. High spatial resolution images of molecules can be obtained with photons or ultrafast electrons. In addition, images of valence molecular orbitals can be extracted via tomographic techniques based on the coherent XUV radiation emitted by a molecular gas exposed to an intense ultra-short infrared laser pulse. In this paper, we demonstrate that similar information can be obtained by inverting energy resolved photoelectron spectra using a simplified analytical model.

Details

Database :
arXiv
Journal :
Phys. Rev. A 94, 023421 (2016)
Publication Type :
Report
Accession number :
edsarx.1607.02273
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevA.94.023421