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Strictly Non-Adiabatic Quantum Control of the Acetylene Dication Using an Infrared Field
- Publication Year :
- 2020
-
Abstract
- We demonstrate the existence of a strictly non-adiabatic control pathway in deprotonation of the acetylene dication. This pathway is identified experimentally by measuring a kinetic energy shift in an ion coincidence experiment. We use a TDSE simulation to identify which properties most strongly affect our control. We find that resonant control around conical intersections is limited by the speed of non-adiabatic dynamics.<br />Comment: 7 pages, 3 figures
- Subjects :
- Physics - Chemical Physics
Quantum Physics
Subjects
Details
- Database :
- arXiv
- Publication Type :
- Report
- Accession number :
- edsarx.2003.02096
- Document Type :
- Working Paper
- Full Text :
- https://doi.org/10.1063/5.0007058