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Symmetry breaking driven by petahertz electron acceleration in a centrosymmetric organic superconductor
- Publication Year :
- 2020
-
Abstract
- Charge acceleration during an intense light field application to solids attracts much attention as elementary processes in high-harmonic generation and photoelectron emission [1-7]. For manipulating such attosecond dynamics of charge, carrier-envelope-phase (CEP:relative phase between carrier oscillation of light field and its envelope function) control has been employed in insulators, nanometal and graphene [8-10]. In superconducting materials, collective control of charge motion is expected because of its strongly coherent nature of quasi-particles. Here, in a layered organic superconductor, second harmonic generation (SHG) is observed by using a single-cycle 6 femtosecond near infrared pulse, which is in contrast to the common belief that even harmonics are forbidden in the centrosymmetric system. The SHG shows a CEP sensitive nature and an enhancement near the superconducting temperature. The result and its quantum many-body analysis indicate that a polarized current is induced by non-dissipative acceleration of charge, which is amplified by superconducting fluctuations. This will lead to petahertz functions of superconductors and of strongly correlated systems.<br />Comment: Anotherversion hase been accepted in Nature communications
- Subjects :
- Condensed Matter - Strongly Correlated Electrons
Subjects
Details
- Database :
- arXiv
- Publication Type :
- Report
- Accession number :
- edsarx.2007.10762
- Document Type :
- Working Paper