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Signatures of a spin-1/2 cooperative paramagnet in the diluted triangular lattice of Y$_2$CuTiO$_6$

Authors :
Kundu, S.
Hossain, Akmal
S, Pranava Keerthi
Das, Ranjan
Baenitz, M.
Baker, Peter J.
Orain, Jean-Christophe
Joshi, D. C.
Mathieu, Roland
Mahadevan, Priya
Pujari, Sumiran
Bhattacharjee, Subhro
Mahajan, A. V.
Sarma, D. D.
Source :
Phys. Rev. Lett. 125, 117206 - Published 9 September 2020
Publication Year :
2020

Abstract

We present a combination of thermodynamic and dynamic experimental signatures of a disorder driven dynamic cooperative paramagnet in a 50% site diluted triangular lattice spin-1/2 system, Y$_2$CuTiO$_6$. Magnetic ordering and spin freezing are absent down to 50 mK, far below the Curie Weiss scale of ~-134 K. We observe scaling collapses of the magnetic field- and temperature-dependent magnetic heat capacity and magnetisation data, respectively, in conformity with expectations from the random singlet physics. Our experiments establish the suppression of any freezing scale, if at all present, by more than three orders of magnitude, opening a plethora of interesting possibilities such as disorder-stabilized long range quantum entangled ground states.<br />Comment: 18 pages, 9 figures, published in Physical Review Letters

Details

Database :
arXiv
Journal :
Phys. Rev. Lett. 125, 117206 - Published 9 September 2020
Publication Type :
Report
Accession number :
edsarx.2009.05137
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevLett.125.117206