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Real-space imaging of acoustic plasmons in large-area CVD graphene

Authors :
Menabde, Sergey G.
Lee, In-Ho
Lee, Sanghyub
Ha, Heonhak
Heiden, Jacob T.
Yoo, Daehan
Kim, Teun-Teun
Lee, Young Hee
Low, Tony
Oh, Sang-Hyun
Jang, Min Seok
Source :
Nature Communications 12, 938 (2021)
Publication Year :
2020

Abstract

An acoustic plasmonic mode in a graphene-dielectric-metal heterostructure has recently been spotlighted as a superior platform for strong light-matter interaction. It originates from the coupling of graphene plasmon with its mirror image and exhibits the largest field confinement in the limit of a nm-thick dielectric. Although recently detected in the far-field regime, optical near-fields of this mode are yet to be observed and characterized. Direct optical probing of the plasmonic fields reflected by the edges of graphene via near-field scattering microscope reveals a relatively small damping rate of the mid-IR acoustic plasmons in our devices, which allows for their real-space mapping even with unprotected, chemically grown, large-area graphene at ambient conditions. We show an acoustic mode that is twice as confined - yet 1.4 times less damped - compared to the graphene surface plasmon under similar conditions. We also image the resonant acoustic Bloch state in a 1D array of gold nanoribbons responsible for the high efficiency of the far-field coupling. Our results highlight the importance of acoustic plasmons as an exceptionally promising platform for large-area graphene-based optoelectronic devices operating in mid-IR.

Details

Database :
arXiv
Journal :
Nature Communications 12, 938 (2021)
Publication Type :
Report
Accession number :
edsarx.2010.01958
Document Type :
Working Paper
Full Text :
https://doi.org/10.1038/s41467-021-21193-5