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Gapless quantum spin liquid in the triangular system Sr$_{3}$CuSb$_{2}$O$_{9}$

Authors :
Kundu, S.
Shahee, Aga
Chakraborty, Atasi
Ranjith, K. M.
Koo, B.
Sichelschmidt, Jörg
Telling, Mark T. F.
Biswas, P. K.
Baenitz, M.
Dasgupta, I.
Pujari, Sumiran
Mahajan, A. V.
Source :
Phys. Rev. Lett. 125, 267202 (2020)
Publication Year :
2020

Abstract

We report gapless quantum spin liquid behavior in the layered triangular Sr$_{3}$CuSb$_{2}$O$_{9}$ (SCSO) system. X-ray diffraction shows superlattice reflections associated with atomic site ordering into triangular Cu planes well-separated by Sb planes. Muon spin relaxation ($\mu$SR) measurements show that the $S = \frac{1}{2}$ moments at the magnetically active Cu sites remain dynamic down to 65 mK in spite of a large antiferromagnetic exchange scale evidenced by a large Curie-Weiss temperature $\theta_{\mathrm{cw}} \simeq $ -143 K as extracted from the bulk susceptibility. Specific heat measurements also show no sign of long-range order down to 0.35 K. The magnetic specific heat ($\mathit{C}$$_{\mathrm{m}}$) below 5 K reveals a $\mathit{C}$$_{\mathrm{m}}$ $=$ $\gamma T$ + $\alpha T$$^{2}$ behavior. The significant $T$$^{2}$ contribution to the magnetic specific heat invites a phenomenology in terms of the so-called Dirac spinon excitations with a linear dispersion. From the low-$T$ specific heat data, we estimate the dominant exchange scale to be $\sim $ 36 K using a Dirac spin liquid ansatz which is not far from the values inferred from microscopic density functional theory calculations ($\sim $ 45 K) as well as high-temperature susceptibility analysis ($\sim$ 70 K). The linear specific heat coefficient is about 18 mJ/mol-K$^2$ which is somewhat larger than for typical Fermi liquids.<br />Comment: 16 pages, 21 figures, including supplementary material. A $S = \frac{1}{2}$ Dirac spin liquid scenario has been put forward to explain the field-dependent specific heat data. Comments are welcome

Details

Database :
arXiv
Journal :
Phys. Rev. Lett. 125, 267202 (2020)
Publication Type :
Report
Accession number :
edsarx.2012.01239
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevLett.125.267202