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Gapless quantum spin liquid in the triangular system Sr$_{3}$CuSb$_{2}$O$_{9}$
- Source :
- Phys. Rev. Lett. 125, 267202 (2020)
- Publication Year :
- 2020
-
Abstract
- We report gapless quantum spin liquid behavior in the layered triangular Sr$_{3}$CuSb$_{2}$O$_{9}$ (SCSO) system. X-ray diffraction shows superlattice reflections associated with atomic site ordering into triangular Cu planes well-separated by Sb planes. Muon spin relaxation ($\mu$SR) measurements show that the $S = \frac{1}{2}$ moments at the magnetically active Cu sites remain dynamic down to 65 mK in spite of a large antiferromagnetic exchange scale evidenced by a large Curie-Weiss temperature $\theta_{\mathrm{cw}} \simeq $ -143 K as extracted from the bulk susceptibility. Specific heat measurements also show no sign of long-range order down to 0.35 K. The magnetic specific heat ($\mathit{C}$$_{\mathrm{m}}$) below 5 K reveals a $\mathit{C}$$_{\mathrm{m}}$ $=$ $\gamma T$ + $\alpha T$$^{2}$ behavior. The significant $T$$^{2}$ contribution to the magnetic specific heat invites a phenomenology in terms of the so-called Dirac spinon excitations with a linear dispersion. From the low-$T$ specific heat data, we estimate the dominant exchange scale to be $\sim $ 36 K using a Dirac spin liquid ansatz which is not far from the values inferred from microscopic density functional theory calculations ($\sim $ 45 K) as well as high-temperature susceptibility analysis ($\sim$ 70 K). The linear specific heat coefficient is about 18 mJ/mol-K$^2$ which is somewhat larger than for typical Fermi liquids.<br />Comment: 16 pages, 21 figures, including supplementary material. A $S = \frac{1}{2}$ Dirac spin liquid scenario has been put forward to explain the field-dependent specific heat data. Comments are welcome
- Subjects :
- Condensed Matter - Strongly Correlated Electrons
Subjects
Details
- Database :
- arXiv
- Journal :
- Phys. Rev. Lett. 125, 267202 (2020)
- Publication Type :
- Report
- Accession number :
- edsarx.2012.01239
- Document Type :
- Working Paper
- Full Text :
- https://doi.org/10.1103/PhysRevLett.125.267202