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Hot electron cooling in InSb probed by ultrafast time-resolved terahertz cyclotron resonance

Authors :
Xia, Chelsea Q.
Monti, Maurizio
Boland, Jessica L.
Herz, Laura M.
Lloyd-Hughes, James
Filip, Marina R.
Johnston, Michael B.
Source :
Phys. Rev. B, 2021, 103, 245205
Publication Year :
2021

Abstract

Measuring terahertz (THz) conductivity on an ultrafast time scale is an excellent way to observe charge-carrier dynamics in semiconductors as a function of time after photoexcitation. However, a conductivity measurement alone cannot separate the effects of charge-carrier recombination from effective mass changes as charges cool and experience different regions of the electronic band structure. Here we present a form of time-resolved magneto-THz spectroscopy which allows us to measure cyclotron effective mass on a picosecond time scale. We demonstrate this technique by observing electron cooling in the technologically-significant narrow-bandgap semiconductor indium antimonide (InSb). A significant reduction of electron effective mass from 0.032$m_\mathrm{e}$ to 0.017$m_\mathrm{e}$ is observed in the first 200ps after injecting hot electrons. Measurement of electron effective mass in InSb as a function of photo-injected electron density agrees well with conduction band non-parabolicity predictions from ab initio calculations of the quasiparticle band structure.

Details

Database :
arXiv
Journal :
Phys. Rev. B, 2021, 103, 245205
Publication Type :
Report
Accession number :
edsarx.2109.05241
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevB.103.245205