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Pressure-induced superconductivity in flat-band Kagome compounds Pd$_3$P$_2$(S$_{1-x}$Se$_x$)$_8$
- Publication Year :
- 2022
-
Abstract
- We performed high-pressure transport studies on the flat-band Kagome compounds, Pd$_3$P$_2$(S$_{1-x}$Se$_x$)$_8$ ($x$ = 0, 0.25), with a diamond anvil cell. For both compounds, the resistivity exhibits an insulating behavior with pressure up to 17 GPa. With pressure above 20 GPa, a metallic behavior is observed at high temperatures in Pd$_3$P$_2$S$_8$, and superconductivity emerges at low temperatures. The onset temperature of superconducting transition $T_{\rm C}$ rises monotonically from 2 K to 4.8 K and does not saturate with pressure up to 43 GPa. For the Se-doped compound Pd$_3$P$_2$(S$_{0.75}$Se$_{0.25}$)$_8$, the $T_{\rm C}$ is about 1.5 K higher than that of the undoped one over the whole pressure range, and reaches 6.4 K at 43 GPa. The upper critical field with field applied along the $c$ axis at typical pressures is about 50$\%$ of the Pauli limit, suggesting a 3D superconductivity. The Hall coefficient in the metallic phase is low and exhibits a peaked behavior at about 30 K, which suggests either a multi-band electronic structure or an electron correlation effect in the system.<br />Comment: 6 pages, 5 figures
- Subjects :
- Condensed Matter - Superconductivity
Subjects
Details
- Database :
- arXiv
- Publication Type :
- Report
- Accession number :
- edsarx.2203.15957
- Document Type :
- Working Paper
- Full Text :
- https://doi.org/10.1088/0256-307X/39/6/067404