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Electrical switching of ferro-rotational order in nano-thick 1T-TaS$_2$ crystals

Authors :
Liu, Gan
Qiu, Tianyu
He, Kuanyu
Liu, Yizhou
Lin, Dongjing
Ma, Zhen
Huang, Zhentao
Tang, Wenna
Xu, Jie
Watanabe, Kenji
Taniguchi, Takashi
Gao, Libo
Wen, Jinsheng
Liu, Jun-Ming
Yan, Binghai
Xi, Xiaoxiang
Source :
Nature Nanotechnology 18, 854-860 (2023)
Publication Year :
2022

Abstract

Hysteretic switching of domain states is a salient character of all ferroic materials and the foundation for their multifunctional applications. Ferro-rotational order is emerging as a new type of ferroic order featuring structural rotations, but its controlled switching remains elusive due to its invariance under both time reversal and spatial inversion. Here, we demonstrate electrical switching of ferro-rotational domain states in nanometer-thick 1T-TaS$_2$ crystals in its charge-density-wave phases. Cooling from the high-symmetry phase to the ferro-rotational phase under an external electric field induces domain state switching and domain wall formation, realized in a simple two-terminal configuration using a volt-scale voltage. Although the electric field does not couple with the order due to symmetry mismatch, it drives domain wall propagation to give rise to reversible, durable, and nonvolatile isothermal state switching at room temperature. These results pave the path for manipulation of the ferro-rotational order and its nanoelectronic applications.

Details

Database :
arXiv
Journal :
Nature Nanotechnology 18, 854-860 (2023)
Publication Type :
Report
Accession number :
edsarx.2211.08782
Document Type :
Working Paper
Full Text :
https://doi.org/10.1038/s41565-023-01403-5