Back to Search Start Over

Electrical control of hybrid exciton transport in a van der Waals heterostructure

Authors :
Tagarelli, Fedele
Lopriore, Edoardo
Erkensten, Daniel
Perea-Causín, Raül
Brem, Samuel
Hagel, Joakim
Sun, Zhe
Pasquale, Gabriele
Watanabe, Kenji
Taniguchi, Takashi
Malic, Ermin
Kis, Andras
Source :
Nature Photonics 17, 615 (2023)
Publication Year :
2023

Abstract

Interactions between out-of-plane dipoles in bosonic gases enable the long-range propagation of excitons. The lack of direct control over collective dipolar properties has hitherto limited the degrees of tunability and the microscopic understanding of exciton transport. In this work, we modulate the layer hybridization and interplay between many-body interactions of excitons in a van der Waals heterostructure with an applied vertical electric field. By performing spatiotemporally resolved measurements supported by microscopic theory, we uncover the dipole-dependent properties and transport of excitons with different degrees of hybridization. Moreover, we find constant emission quantum yields of the transporting species as a function of excitation power with dominating radiative decay mechanisms over nonradiative ones, a fundamental requirement for efficient excitonic devices. Our findings provide a complete picture of the many-body effects in the transport of dilute exciton gases and have crucial implications for the study of emerging states of matter, such as Bose-Einstein condensation, as well as for optoelectronic applications based on exciton propagation.

Details

Database :
arXiv
Journal :
Nature Photonics 17, 615 (2023)
Publication Type :
Report
Accession number :
edsarx.2303.00419
Document Type :
Working Paper
Full Text :
https://doi.org/10.1038/s41566-023-01198-w