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Directed Autonomous Motion and Chiral Separation of Self-Propelled Janus Particles in Convection Roll Arrays

Authors :
Bag, Poulami
Nayak, Shubhadip
Debnath, Tanwi
Ghosh, Pulak K.
Source :
J. Phys. Chem. Lett. 2022, 13, 11413
Publication Year :
2023

Abstract

Self-propelled Janus particles exhibit autonomous motion thanks to engines of their own. However, due to randomly changing direction of such motion they are of little use for emerging nano-technological and bio-medical applications. Here, we numerically show that the motion of chiral active Janus can be directed subjecting them to a linear array of convection rolls. Rectification power of self-propulsion motion here can be made more than 60% which is much larger than earlier reports. We show that rectification of chiral Janus particle's motion leads to conspicuous segregation of dextrogyre and levogyre active particles from a racemic binary mixture. Further, we demonstrate how efficiently the rectification effect can be exploited to separate dextrogyre and levogyre particles when their intrinsic torques are distributed with Gaussian statistics.

Details

Database :
arXiv
Journal :
J. Phys. Chem. Lett. 2022, 13, 11413
Publication Type :
Report
Accession number :
edsarx.2303.14698
Document Type :
Working Paper
Full Text :
https://doi.org/10.1021/acs.jpclett.2c03193