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Long-lasting XUV activation of helium nanodroplets for avalanche ionization

Authors :
Medina, C.
Lægdsmand, A. Ø.
Ltaief, L. Ben
Hoque, Z.
Roos, A. H.
Jurkovič, M.
Hort, O.
Finke, O.
Albrecht, M.
Nejdl, J.
Stienkemeier, F.
Andreasson, J.
Klimešová, E.
Krikunova, M.
Heidenreich, A.
Mudrich, M.
Publication Year :
2023

Abstract

We study the dynamics of avalanche ionization of pure helium nanodroplets activated by a weak extreme-ultraviolet (XUV) pulse and driven by an intense near-infrared (NIR) pulse. In addition to a transient enhancement of ignition of a nanoplasma at short delay times $\sim200$~fs, long-term activation of the nanodroplets lasting up to a few nanoseconds is observed. Molecular dynamics simulations suggest that the short-term activation is caused by the injection of seed electrons into the droplets by XUV photoemission. Long-term activation appears due to electrons remaining loosely bound to photoions which form stable `snowball' structures in the droplets. Thus, we show that XUV irradiation can induce long-lasting changes of the strong-field optical properties of nanoparticles, potentially opening new routes to controlling avalanche-ionization phenomena in nanostructures and condensed-phase systems.

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.2304.06374
Document Type :
Working Paper
Full Text :
https://doi.org/10.1088/1367-2630/acd5f6