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Disorder-enriched magnetic excitations in the Kitaev quantum spin liquid candidate Na$_2$Co$_2$TeO$_6$

Authors :
Xiang, Li
Dhakal, Ramesh
Ozerov, Mykhaylo
Jiang, Yuxuan
Mou, Banasree S.
Ozarowski, Andrzej
Huang, Qing
Zhou, Haidong
Fang, Jiyuan
Winter, Stephen M.
Jiang, Zhigang
Smirnov, Dmitry
Publication Year :
2023

Abstract

Using optical magneto-spectroscopy, we investigate the magnetic excitations of Na$_2$Co$_2$TeO$_6$ in a broad magnetic field range ($0\ \rm{T}\leq B\leq 17.5\ \rm{T}$) at low temperature. Our measurements reveal rich spectra of in-plane magnetic excitations with a surprisingly large number of modes, even in the high-field spin-polarized state. Theoretical calculations find that the Na-occupation disorder in \NCTO plays a crucial role in generating these modes. Our work demonstrates the necessity to consider disorder in the spin environment in the search for Kitaev quantum spin liquid states in practicable materials.

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.2305.07734
Document Type :
Working Paper