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Formation and Dissociation of Field-Linked Tetramers
- Publication Year :
- 2024
-
Abstract
- We investigate the static and dynamic properties of tetratomic molecules formed by two microwave-shielded polar molecules across field-linked resonances. In particular, we focus on two-body physics and experimental techniques unexplored in the recent experiment [X.-Y. Chen {\it et al}., Nature {\bf626}, 283 (2024)]. We show that, compared to the lowest tetramer state, higher tetramer states typically have longer lifetimes, which may facilitate a further cooling of tetramer gases towards quantum degeneracy. To detect tetramers, we identify the distinctive time-of-flight images from ramp dissociation, which can be observed by lowering the ramp rate of the microwave. Remarkably, in the modulational dissociation of tetramers, we find that multi-photon processes induce dissociation even below the threshold modulation frequency when the modulation amplitude is sufficiently high. Given the universal form of the inter-molecular potential for microwave-shielded polar molecules, our results also apply to other molecular gases widely explored in recent experiments.
- Subjects :
- Quantum Physics
Subjects
Details
- Database :
- arXiv
- Publication Type :
- Report
- Accession number :
- edsarx.2405.13645
- Document Type :
- Working Paper