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High-quality full-color carbon quantum dots synthesized under an unprecedentedly mild condition

High-quality full-color carbon quantum dots synthesized under an unprecedentedly mild condition

Authors :
Yuan-Jun Tong
Lu-Dan Yu
Yanjun Huang
Yutong Li
Nan Li
Qi Fu
Yu-Xin Ye
Fang Zhu
Janusz Pawliszyn
Jianqiao Xu
Gangfeng Ouyang
Source :
iScience, Vol 25, Iss 6, Pp 104421- (2022)
Publication Year :
2022
Publisher :
Elsevier, 2022.

Abstract

Summary: Carbon quantum dots (CQDs) are highly promising to be applied in light-emitting, chemosensing, and other cutting-edge domains. Herein, we successfully fabricate high-quality full-color CQDs under unprecedentedly low temperature and pressure (85°C, 1.88 bar). Stable and narrow fluorescent emissions ranging from blue to green and red light were realized by simple amine engineering, which were further mixed into white-light CQDs with the absolute photoluminescent quantum yield reaching 19.2%. The average mass yield of the CQDs reached 69.0%. The optical performances demonstrated that the CQDs possessed uniform luminescent centers and dominant radiative decay channels. Component analysis further suggested that dehydrated condensation between carboxyl and amine groups directed the growth of the CQDs. By utilizing the CQDs, full-color light-emitting diodes and logic gate sensors were developed. This study paves an important step for promoting the application of CQDs by providing an energy-efficient, safe, and productive synthetic strategy.

Details

Language :
English
ISSN :
25890042
Volume :
25
Issue :
6
Database :
Directory of Open Access Journals
Journal :
iScience
Publication Type :
Academic Journal
Accession number :
edsdoj.2aa0e2d4290e4607bf8aaecf548ed67e
Document Type :
article
Full Text :
https://doi.org/10.1016/j.isci.2022.104421