Back to Search Start Over

Real-space perspective on dephasing in solid-state high harmonic generation

Authors :
Graham G. Brown
Álvaro Jiménez-Galán
Rui E. F. Silva
Misha Ivanov
Source :
Physical Review Research, Vol 6, Iss 4, p 043005 (2024)
Publication Year :
2024
Publisher :
American Physical Society, 2024.

Abstract

We develop and demonstrate a fully real-space perspective on high harmonic generation (HHG) in crystals. Due to the Wannier-Stark localization induced on subcycle timescales in the presence of a strong field, real-space descriptions are natural for strongly driven solids. Our approach allows us to address the origin of the extremely short dephasing times, which appear necessary for agreement between experimental HHG measurements and theoretical calculations generally performed in reciprocal space. We develop a physically transparent model of real-space dephasing which relates its rate to the distance between different sites in a laser-driven lattice. Our approach leads to well-structured high harmonic spectra at the microscopic level, reproduces the results of macroscopic propagation, and demonstrates that the requirement for ultrafast dephasing times stems from the need for suppressing recombination events with large electron-hole separations during radiative recombination.

Subjects

Subjects :
Physics
QC1-999

Details

Language :
English
ISSN :
26431564
Volume :
6
Issue :
4
Database :
Directory of Open Access Journals
Journal :
Physical Review Research
Publication Type :
Academic Journal
Accession number :
edsdoj.2c0cf10603f24e6fb88c8eb38141dc98
Document Type :
article
Full Text :
https://doi.org/10.1103/PhysRevResearch.6.043005