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Nonreciprocal linear dichroism observed in electron spin resonance spectra of the magnetoelectric multiferroic Pb(TiO)Cu_{4}(PO_{4})_{4}

Authors :
Mitsuru Akaki
Kenta Kimura
Yasuyuki Kato
Yuya Sawada
Yasuo Narumi
Hitoshi Ohta
Tsuyoshi Kimura
Yukitoshi Motome
Masayuki Hagiwara
Source :
Physical Review Research, Vol 3, Iss 4, p L042043 (2021)
Publication Year :
2021
Publisher :
American Physical Society, 2021.

Abstract

It is known that magnetic excitations in magnetoelectric multiferroics can be induced by the oscillation of electric polarization, called electromagnons, which often cause nonreciprocal optical phenomena. Energy diagrams of the excitations in the magnetoelectric multiferroic Pb(TiO)Cu_{4}(PO_{4})_{4} were obtained in wide ranges of magnetic fields up to 50 T and frequencies below 2 THz. Some of the observed resonance modes were reproduced qualitatively by a numerical analysis based on the generalized spin-wave theory. Moreover, we found that electron spin resonance (ESR) signals on some of the modes can be modulated by applying an electric field. This result implies the presence of nonreciprocal linear dichroism on the ESR signals in Pb(TiO)Cu_{4}(PO_{4})_{4}.

Subjects

Subjects :
Physics
QC1-999

Details

Language :
English
ISSN :
26431564
Volume :
3
Issue :
4
Database :
Directory of Open Access Journals
Journal :
Physical Review Research
Publication Type :
Academic Journal
Accession number :
edsdoj.72d841b81b244835b180283f868b754d
Document Type :
article
Full Text :
https://doi.org/10.1103/PhysRevResearch.3.L042043